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High-resolution transient and permanent spectral hole burning in Ce3+ : Y2SiO5 at liquid helium temperatures
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- Karlsson, Jenny (author)
- Lund University,Lunds universitet,Atomfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Atomic Physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH,PSL University
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- Nilsson, Adam N. (author)
- Lund University,Lunds universitet,Atomfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Atomic Physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH
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- Serrano, Diana (author)
- Lund University,Lunds universitet,Atomfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Atomic Physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH,University of Zurich
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- 2016
- 2016
- English.
- In: Physical Review B. - 1098-0121. ; 93:22
- Journal article (peer-reviewed)
Abstract
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- We perform hole burning with a low-drift stabilized laser within the zero phonon line of the 4f-5d transition in Ce3+:Y2SiO5 at 2 K. The narrowest spectral holes appear for small applied magnetic fields and are 6±4 MHz wide (FWHM). This puts an upper bound on the homogeneous linewidth of the transition to 3±2 MHz, which is close to lifetime limited. The spin level relaxation time is measured to 72±21 ms with a magnetic field of 10 mT. A slow permanent hole burning mechanism is observed. If the excitation frequency is not changed the fluorescence intensity is reduced by more than 50% after a couple of minutes of continuous excitation. The spectral hole created by the permanent hole burning has a width in the tens of MHz range, which indicates that a trapping mechanism occurs via the 5d state.
Subject headings
- NATURVETENSKAP -- Fysik -- Den kondenserade materiens fysik (hsv//swe)
- NATURAL SCIENCES -- Physical Sciences -- Condensed Matter Physics (hsv//eng)
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- Karlsson, Jenny
- Nilsson, Adam N.
- Serrano, Diana
- Walther, Andreas
- Goldner, Philipp ...
- Ferrier, Alban
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- Rippe, Lars
- Kröll, Stefan
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