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Rydberg-Resolved Resonant Inelastic Soft X-Ray Scattering: Dynamics at Core Ionization Thresholds

Rubensson, Jan-Erik (author)
Uppsala universitet,Uppsala University,Molekyl- och kondenserade materiens fysik
Söderström, Johan (author)
Uppsala universitet,Uppsala University,Molekyl- och kondenserade materiens fysik
Binggeli, Christian (author)
Uppsala universitet,Uppsala University,Institutionen för fysik och astronomi
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Gråsjö, Johan (author)
Uppsala universitet,Uppsala University,Institutionen för farmaci
Andersson, Joakim (author)
Uppsala universitet,Uppsala University,National University of Singapore,Molekyl- och kondenserade materiens fysik
Såthe, Conny (author)
Lund University,Lunds universitet,MAX IV-laboratoriet,MAX IV Laboratory
Hennies, Franz (author)
Lund University,Lunds universitet,MAX IV-laboratoriet,MAX IV Laboratory
Bisogni, V. (author)
Paul Scherrer Institute
Huang, Y. (author)
Paul Scherrer Institute
Olalde, P. (author)
Paul Scherrer Institute
Schmitt, T. (author)
Paul Scherrer Institute
Strocov, V. N. (author)
Paul Scherrer Institute
Föhlisch, A. (author)
Helmholtz Association of German Research Centers,University of Potsdam
Kennedy, B. (author)
Helmholtz Association of German Research Centers
Pietzsch, A. (author)
Helmholtz Association of German Research Centers
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 (creator_code:org_t)
2015
2015
English.
In: Physical Review Letters. - 1079-7114 .- 0031-9007. ; 114:13
Related links:
http://dx.doi.org/10...
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https://lup.lub.lu.s...
https://doi.org/10.1...
https://urn.kb.se/re...
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  • Journal article (peer-reviewed)
Abstract Subject headings
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  • Resonant inelastic x-ray scattering spectra excited in the immediate vicinity of the core-level ionization thresholds of N-2 have been recorded. Final states of well-resolved symmetry-selected Rydberg series converging to valence-level ionization thresholds with vibrational excitations are observed. The results are well described by a quasi-two-step model which assumes that the excited electron is unaffected by the radiative decay. This threshold dynamics simplifies the interpretation of resonant inelastic x-ray scattering spectra considerably and facilitates characterization of low-energy excited final states in molecular systems.

Subject headings

NATURVETENSKAP  -- Fysik (hsv//swe)
NATURAL SCIENCES  -- Physical Sciences (hsv//eng)

Publication and Content Type

art (subject category)
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