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Time-resolved photo...
Time-resolved photoelectron imaging of complex resonances in molecular nitrogen
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- Fushitani, Mizuho (author)
- Nagoya University
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- Pratt, Stephen T. (author)
- Argonne National Laboratory
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- You, Daehyun (author)
- Tohoku University
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- Saito, Shu (author)
- Tohoku University
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- Luo, Yu (author)
- Tohoku University
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- Ueda, Kiyoshi (author)
- Tohoku University
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- Fujise, Hikaru (author)
- Nagoya University
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- Hishikawa, Akiyoshi (author)
- Nagoya University
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- Ibrahim, Heide (author)
- Institut National de la Recherche Scientifique
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- Légaré, François (author)
- Institut National de la Recherche Scientifique
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- Johnsson, Per (author)
- Lund University,Lunds universitet,Atomfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Atomic Physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH
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- Peschel, Jasper (author)
- Lund University,Lunds universitet,Atomfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Atomic Physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH
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- Simpson, Emma R. (author)
- Lund University,Lunds universitet,Atomfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Atomic Physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH
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- Olofsson, Anna (author)
- Lund University,Lunds universitet,Atomfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Atomic Physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH
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- Mauritsson, Johan (author)
- Lund University,Lunds universitet,Atomfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Atomic Physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH
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- Carpeggiani, Paolo Antonio (author)
- Technical University Vienna (TU Wien)
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- Maroju, Praveen Kumar (author)
- Albert-Ludwigs University Freiburg
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- Moioli, Matteo (author)
- Albert-Ludwigs University Freiburg
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- Ertel, Dominik (author)
- Albert-Ludwigs University Freiburg
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- Shah, Ronak (author)
- Albert-Ludwigs University Freiburg
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- Sansone, Giuseppe (author)
- Albert-Ludwigs University Freiburg
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- Csizmadia, Tamás (author)
- ELI-HU Non-profit Ltd
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- Dumergue, Mathieu (author)
- ELI-HU Non-profit Ltd
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- Harshitha, N. G. (author)
- ELI-HU Non-profit Ltd
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- Kühn, Sergei (author)
- ELI-HU Non-profit Ltd
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- Callegari, Carlo (author)
- Elettra Sincrotrone Trieste
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- Plekan, Oksana (author)
- Elettra Sincrotrone Trieste
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- Di Fraia, Michele (author)
- Elettra Sincrotrone Trieste
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- Danailov, Miltcho B. (author)
- Elettra Sincrotrone Trieste
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- Demidovich, Alexander (author)
- Elettra Sincrotrone Trieste
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- Giannessi, Luca (author)
- Elettra Sincrotrone Trieste,INFN Frascati National Laboratory
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- Raimondi, Lorenzo (author)
- Elettra Sincrotrone Trieste
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- Zangrando, Marco (author)
- Elettra Sincrotrone Trieste,CNR Istituto Officina dei Materiali (IOM)
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- De Ninno, Giovanni (author)
- Elettra Sincrotrone Trieste,University of Nova Gorica
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- Ribič, Primož Rebernik (author)
- Elettra Sincrotrone Trieste,University of Nova Gorica
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- Prince, Kevin C. (author)
- Swinburne University of Technology,Elettra Sincrotrone Trieste
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(creator_code:org_t)
- AIP Publishing, 2021
- 2021
- English 14 s.
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In: The Journal of chemical physics. - : AIP Publishing. - 0021-9606 .- 1089-7690. ; 154:14
- Related links:
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http://dx.doi.org/10...
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https://lup.lub.lu.s...
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https://doi.org/10.1...
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Abstract
Subject headings
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- We have used the FERMI free-electron laser to perform time-resolved photoelectron imaging experiments on a complex group of resonances near 15.38 eV in the absorption spectrum of molecular nitrogen, N2, under jet-cooled conditions. The new data complement and extend the earlier work of Fushitani et al. [Opt. Express 27, 19702–19711 (2019)], who recorded time-resolved photoelectron spectra for this same group of resonances. Time-dependent oscillations are observed in both the photoelectron yields and the photoelectron angular distributions, providing insight into the interactions among the resonant intermediate states. In addition, for most states, we observe an exponential decay of the photoelectron yield that depends on the ionic final state. This observation can be rationalized by the different lifetimes for the intermediate states contributing to a particular ionization channel. Although there are nine resonances within the group, we show that by detecting individual photoelectron final states and their angular dependence, we can identify and differentiate quantum pathways within this complex system.
Subject headings
- NATURVETENSKAP -- Fysik -- Atom- och molekylfysik och optik (hsv//swe)
- NATURAL SCIENCES -- Physical Sciences -- Atom and Molecular Physics and Optics (hsv//eng)
Publication and Content Type
- art (subject category)
- ref (subject category)
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- By the author/editor
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Fushitani, Mizuh ...
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Pratt, Stephen T ...
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You, Daehyun
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Saito, Shu
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Luo, Yu
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Ueda, Kiyoshi
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show more...
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Fujise, Hikaru
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Hishikawa, Akiyo ...
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Ibrahim, Heide
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Légaré, François
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Johnsson, Per
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Peschel, Jasper
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Simpson, Emma R.
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Olofsson, Anna
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Mauritsson, Joha ...
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Carpeggiani, Pao ...
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Maroju, Praveen ...
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Moioli, Matteo
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Ertel, Dominik
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Shah, Ronak
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Sansone, Giusepp ...
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Csizmadia, Tamás
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Dumergue, Mathie ...
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Harshitha, N. G.
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Kühn, Sergei
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Callegari, Carlo
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Plekan, Oksana
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Di Fraia, Michel ...
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Danailov, Miltch ...
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Demidovich, Alex ...
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Giannessi, Luca
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Raimondi, Lorenz ...
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Zangrando, Marco
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De Ninno, Giovan ...
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Ribič, Primož Re ...
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Prince, Kevin C.
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- About the subject
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- NATURAL SCIENCES
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NATURAL SCIENCES
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and Physical Science ...
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and Atom and Molecul ...
- Articles in the publication
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The Journal of c ...
- By the university
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Lund University