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Spectroscopic chara...
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Chiu, Chun-ChienNational Cheng Kung University
(author)
Spectroscopic characterization of electronic structures of ultra-thin single crystal La0.7Sr0.3MnO3
- Article/chapterEnglish2021
Publisher, publication year, extent ...
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2021-03-04
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Springer Science and Business Media LLC,2021
Numbers
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LIBRIS-ID:oai:lup.lub.lu.se:981ea70f-fb53-4661-b413-b2be64047840
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https://lup.lub.lu.se/record/981ea70f-fb53-4661-b413-b2be64047840URI
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https://doi.org/10.1038/s41598-021-84598-8DOI
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Language:English
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Summary in:English
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Subject category:art swepub-publicationtype
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Subject category:ref swepub-contenttype
Notes
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We have successfully fabricated high quality single crystalline La0.7Sr0.3MnO3 (LSMO) film in the freestanding form that can be transferred onto silicon wafer and copper mesh support. Using soft x-ray absorption (XAS) and resonant inelastic x-ray scattering (RIXS) spectroscopy in transmission and reflection geometries, we demonstrate that the x-ray emission from Mn 3s-2p core-to-core transition (3sPFY) seen in the RIXS maps can represent the bulk-like absorption signal with minimal self-absorption effect around the Mn L3-edge. Similar measurements were also performed on a reference LSMO film grown on the SrTiO3 substrate and the agreement between measurements substantiates the claim that the bulk electronic structures can be preserved even after the freestanding treatment process. The 3sPFY spectrum obtained from analyzing the RIXS maps offers a powerful way to probe the bulk electronic structures in thin films and heterostructures when recording the XAS spectra in the transmission mode is not available.
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Chang, Yao-WenNational Cheng Kung University
(author)
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Shao, Yu-ChengLawrence Berkeley National Laboratory
(author)
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Liu, Yu-ChenNational Cheng Kung University
(author)
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Lee, Jenn-MinLund University,Lunds universitet,MAX IV-laboratoriet,MAX IV Laboratory(Swepub:lu)je6687le
(author)
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Huang, Shih-WenLund University,Lunds universitet,MAX IV-laboratoriet,MAX IV Laboratory(Swepub:lu)maxl-sha
(author)
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Yang, WanliLawrence Berkeley National Laboratory
(author)
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Guo, JinghuaLawrence Berkeley National Laboratory
(author)
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de Groot, Frank M. F.Utrecht University
(author)
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Yang, Jan-ChiNational Cheng Kung University
(author)
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Chuang, Yi-DeLawrence Berkeley National Laboratory
(author)
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National Cheng Kung UniversityLawrence Berkeley National Laboratory
(creator_code:org_t)
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In:Scientific Reports: Springer Science and Business Media LLC112045-2322
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Chiu, Chun-Chien
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Chang, Yao-Wen
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Shao, Yu-Cheng
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Liu, Yu-Chen
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Lee, Jenn-Min
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Huang, Shih-Wen
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Yang, Wanli
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Guo, Jinghua
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de Groot, Frank ...
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Yang, Jan-Chi
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Chuang, Yi-De
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- NATURAL SCIENCES
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NATURAL SCIENCES
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Lund University