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From localised to delocalised electronic states in free Ar, Kr and Xe clusters

Feifel, Raimund (author)
Uppsala universitet,Fysik V,Fysik II
Tchaplyguine, Maxim (author)
Lund University,Lunds universitet,MAX IV-laboratoriet,MAX IV Laboratory
Öhrwall, Gunnar (author)
Uppsala universitet,Fysiska institutionen,Fysik V,Fysik II
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Salonen, M (author)
Lundwall, Marcus (author)
Uppsala universitet,Fysiska institutionen,Fysik V,Fysik II
Marinho, Ricardo (author)
Uppsala universitet,Fysik V,Fysik II
Gisselbrecht, Mathieu (author)
Lund University,Lunds universitet,Synkrotronljusfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Synchrotron Radiation Research,Department of Physics,Departments at LTH,Faculty of Engineering, LTH
Ristinmaa Sörensen, Stacey (author)
Lund University,Lunds universitet,Synkrotronljusfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Synchrotron Radiation Research,Department of Physics,Departments at LTH,Faculty of Engineering, LTH
de Brito, AN (author)
Karlsson, Leif (author)
Uppsala universitet,Fysiska institutionen,Fysik V,Fysik II,Fysik 2
Mårtensson, Nils (author)
Uppsala universitet,Fysiska institutionen,Fysik V,Fysik II
Svensson, Svante (author)
Uppsala universitet,Fysiska institutionen,Fysik V,Fysik II
Björneholm, Olle (author)
Uppsala universitet,Fysiska institutionen,Fysik V,Fysik II
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 (creator_code:org_t)
Springer Science and Business Media LLC, 2004
2004
English.
In: European Physical Journal D. Atomic, Molecular, Optical and Plasma Physics. - : Springer Science and Business Media LLC. - 1434-6060 .- 1434-6079. ; 30:3, s. 343-351
Related links:
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  • Journal article (peer-reviewed)
Abstract Subject headings
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  • We present new results for the inner valence levels of clusters of the three inert gases Ar, Kr and Xe based on photoelectron spectroscopy studies. The inner valence levels are compared to the localised core levels and to the delocalised outer valence levels. This comparison shows a gradual change from a relatively localised behaviour for Ar inner valence 3s, over the intermediate case of Kr inner valence 4s, to a more delocalised behaviour for Xe inner valence 5s. This change correlates well with the ratio between the orbital sizes and the interatomic distances. The Kr4s intermediate case is found to exhibit characteristics of both localised and delocalised behaviour.

Subject headings

NATURVETENSKAP  -- Fysik (hsv//swe)
NATURAL SCIENCES  -- Physical Sciences (hsv//eng)
NATURVETENSKAP  -- Fysik -- Atom- och molekylfysik och optik (hsv//swe)
NATURAL SCIENCES  -- Physical Sciences -- Atom and Molecular Physics and Optics (hsv//eng)

Publication and Content Type

art (subject category)
ref (subject category)

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