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The Kinetic Energy ...
The Kinetic Energy of PAH Dication and Trication Dissociation Determined by Recoil-Frame Covariance Map Imaging
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- Lee, Jason W.l. (author)
- German Electron Synchrotron (DESY),University of Oxford
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- Tikhonov, Denis (author)
- German Electron Synchrotron (DESY),University of Kiel
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- Allum, Felix (author)
- University of Oxford
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- Boll, Rebecca (author)
- European XFEL GmbH
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- Chopra, Pragya (author)
- German Electron Synchrotron (DESY),University of Kiel
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- Erk, Benjamin (author)
- German Electron Synchrotron (DESY)
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- Gruet, Sébastien (author)
- German Electron Synchrotron (DESY)
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- He, Lanhai (author)
- German Electron Synchrotron (DESY)
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- Heathcote, David (author)
- University of Oxford
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- Kazemi, Mehdi (author)
- German Electron Synchrotron (DESY)
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- Lahl, Jan (author)
- Lund University,Lunds universitet,Atomfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Atomic Physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH
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- Lemmens, Alexander K. (author)
- Radboud University Nijmegen,University of Amsterdam
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- Loru, Donatella (author)
- German Electron Synchrotron (DESY)
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- Maclot, Sylvain (author)
- KTH Royal Institute of Technology,University of Gothenburg
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- Mason, Robert (author)
- University of Oxford
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- Müller, Erland (author)
- German Electron Synchrotron (DESY)
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- Mullins, Terry (author)
- University of Hamburg
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- Passow, Christopher (author)
- German Electron Synchrotron (DESY)
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- Peschel, Jasper (author)
- Lund University,Lunds universitet,Atomfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Atomic Physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH
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- Ramm, Daniel (author)
- German Electron Synchrotron (DESY)
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- Steber, Amanda L (author)
- University of Hamburg,University of Kiel,German Electron Synchrotron (DESY)
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- Bari, Sadia (author)
- German Electron Synchrotron (DESY)
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- Brouard, Mark (author)
- University of Oxford
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- Burt, Michael (author)
- University of Oxford
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- Küpper, Jochen (author)
- German Electron Synchrotron (DESY),University of Hamburg
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- Eng-johnsson, Per (author)
- Lund University,Lunds universitet,Lunds lasercentrum, LLC,Annan verksamhet, LTH,Lunds Tekniska Högskola,Atomfysik,Fysiska institutionen,Institutioner vid LTH,LTH profilområde: Avancerade ljuskällor,LTH profilområden,Lund Laser Centre, LLC,Other operations, LTH,Faculty of Engineering, LTH,Atomic Physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH,LTH Profile Area: Photon Science and Technology,LTH Profile areas,Faculty of Engineering, LTH
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- Rijs, Anouk (author)
- Radboud University Nijmegen
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- Rolles, Daniel (author)
- Kansas State University
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- Vallance, Claire (author)
- University of Oxford
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- Manschwetus, Bastian (author)
- German Electron Synchrotron (DESY)
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- Schnell, Melanie (author)
- German Electron Synchrotron (DESY)
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(creator_code:org_t)
- 2022
- 2022
- English 10 s.
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In: Physical Chemistry Chemical Physics. - 1463-9084. ; 24:38, s. 23096-23105
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http://dx.doi.org/10... (free)
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Abstract
Subject headings
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- We investigated the dissociation of dications and trications of three polycyclic aromatic hydrocarbons (PAHs), fluorene, phenanthrene, and pyrene. PAHs are a family of molecules ubiquitous in space and involved in much of the chemistry of the interstellar medium. In our experiments, ions are formed by interaction with 30.3 nm extreme ultraviolet (XUV) photons, and their velocity map images are recorded using a PImMS2 multi-mass imaging sensor. Application of recoil-frame covariance analysis allows the total kinetic energy release (TKER) associated with multiple fragmentation channels to be determined to high precision, ranging 1.94-2.60 eV and 2.95-5.29 eV for the dications and trications, respectively. Experimental measurements are supported by Born-Oppenheimer molecular dynamics (BOMD) simulations.
Subject headings
- NATURVETENSKAP -- Fysik -- Atom- och molekylfysik och optik (hsv//swe)
- NATURAL SCIENCES -- Physical Sciences -- Atom and Molecular Physics and Optics (hsv//eng)
Publication and Content Type
- art (subject category)
- ref (subject category)
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To the university's database
- By the author/editor
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Lee, Jason W.l.
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Tikhonov, Denis
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Allum, Felix
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Boll, Rebecca
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Chopra, Pragya
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Erk, Benjamin
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show more...
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Gruet, Sébastien
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He, Lanhai
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Heathcote, David
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Kazemi, Mehdi
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Lahl, Jan
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Lemmens, Alexand ...
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Loru, Donatella
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Maclot, Sylvain
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Mason, Robert
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Müller, Erland
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Mullins, Terry
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Passow, Christop ...
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Peschel, Jasper
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Ramm, Daniel
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Steber, Amanda L
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Bari, Sadia
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Brouard, Mark
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Burt, Michael
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Küpper, Jochen
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Eng-johnsson, Pe ...
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Rijs, Anouk
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Rolles, Daniel
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Vallance, Claire
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Manschwetus, Bas ...
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Schnell, Melanie
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show less...
- About the subject
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- NATURAL SCIENCES
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NATURAL SCIENCES
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and Physical Science ...
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and Atom and Molecul ...
- Articles in the publication
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Physical Chemist ...
- By the university
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Lund University