Diesel soot aging in urban plumes within hours under cold dark and humid conditions

Eriksson, Axel (författare): Lund University,Lunds universitet,Ergonomi och aerosolteknologi,Institutionen för designvetenskaper,Institutioner vid LTH,Lunds Tekniska Högskola,Kärnfysik,Fysiska institutionen,Ergonomics and Aerosol Technology,Department of Design Sciences,Departments at LTH,Faculty of Engineering, LTH,Nuclear physics,Department of Physics,Faculty of Engineering, LTH

Wittbom, Cerina (författare): Lund University,Lunds universitet,Kärnfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Nuclear physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH

Roldin, Pontus (författare): Lund University,Lunds universitet,Kärnfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Nuclear physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH,University of Helsinki

Öström, Emilie (författare): Lund University,Lunds universitet,Centrum för miljö- och klimatvetenskap (CEC),Naturvetenskapliga fakulteten,Kärnfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Centre for Environmental and Climate Science (CEC),Faculty of Science,Nuclear physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH

Nilsson, Patrik (författare): Lund University,Lunds universitet,Ergonomi och aerosolteknologi,Institutionen för designvetenskaper,Institutioner vid LTH,Lunds Tekniska Högskola,Ergonomics and Aerosol Technology,Department of Design Sciences,Departments at LTH,Faculty of Engineering, LTH

Martinsson, Johan (författare): Lund University,Lunds universitet,Centrum för miljö- och klimatvetenskap (CEC),Naturvetenskapliga fakulteten,Kärnfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Centre for Environmental and Climate Science (CEC),Faculty of Science,Nuclear physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH

Rissler, Jenny (författare): Lund University,Lunds universitet,Ergonomi och aerosolteknologi,Institutionen för designvetenskaper,Institutioner vid LTH,Lunds Tekniska Högskola,Ergonomics and Aerosol Technology,Department of Design Sciences,Departments at LTH,Faculty of Engineering, LTH

NORDIN, ERIK (författare): Lund University,Lunds universitet,Ergonomi och aerosolteknologi,Institutionen för designvetenskaper,Institutioner vid LTH,Lunds Tekniska Högskola,Ergonomics and Aerosol Technology,Department of Design Sciences,Departments at LTH,Faculty of Engineering, LTH

Svenningsson, Birgitta (författare): Lund University,Lunds universitet,Kärnfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Nuclear physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH

Pagels, Joakim (författare): Lund University,Lunds universitet,Ergonomi och aerosolteknologi,Institutionen för designvetenskaper,Institutioner vid LTH,Lunds Tekniska Högskola,Ergonomics and Aerosol Technology,Department of Design Sciences,Departments at LTH,Faculty of Engineering, LTH

Swietlicki, Erik (författare): Lund University,Lunds universitet,Kärnfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Nuclear physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH

(creator_code:org_t)

2017-09-28
2017
Engelska.
Ingår i: Scientific Reports. - : Springer Science and Business Media LLC. - 2045-2322.

Relaterad länk:: http://dx.doi.org/10... (free); visa fler...; https://doi.org/10.1...; https://lup.lub.lu.s...; https://doi.org/10.1...; visa färre...

Abstract Ämnesord

Stäng

Fresh and aged diesel soot particles have different impacts on climate and human health. While fresh diesel soot particles are highly aspherical and non-hygroscopic, aged particles are spherical and hygroscopic. Aging and its effect on water uptake also controls the dispersion of diesel soot in the atmosphere. Understanding the timescales on which diesel soot ages in the atmosphere is thus important, yet knowledge thereof is lacking. We show that under cold, dark and humid conditions the atmospheric transformation from fresh to aged soot occurs on a timescale of less than five hours. Under dry conditions in the laboratory, diesel soot transformation is much less efficient. While photochemistry drives soot aging, our data show it is not always a limiting factor. Field observations together with aerosol process model simulations show that the rapid ambient diesel soot aging in urban plumes is caused by coupled ammonium nitrate formation and water uptake.

Fresh and aged diesel soot particles have different impacts on climate and human health. Whilefresh diesel soot particles are highly aspherical and non-hygroscopic, aged particles are sphericaland hygroscopic. Aging and its effect on water uptake also controls the dispersion of diesel soot inthe atmosphere. Understanding the timescales on which diesel soot ages in the atmosphere is thus important, yet knowledge thereof is lacking. We show that under cold, dark and humid conditions the atmospheric transformation from fresh to aged soot occurs on a timescale of less than five hours. Under dry conditions in the laboratory, diesel soot transformation is much less efficient. While photochemistry drives soot aging, our data show it is not always a limiting factor. Field observations together with aerosol process model simulations show that the rapid ambient diesel soot aging in urban plumes is caused by coupled ammonium nitrate formation and water uptake

Av författaren/redakt...: Eriksson, Axel; Wittbom, Cerina; Roldin, Pontus; Sporre, Moa; Öström, Emilie; Nilsson, Patrik; visa fler...; Martinsson, Joha ...; Rissler, Jenny; NORDIN, ERIK; Svenningsson, Bi ...; Pagels, Joakim; Swietlicki, Erik; visa färre...

Om ämnet

NATURVETENSKAP: NATURVETENSKAP; och Geovetenskap och ...; och Miljövetenskap

NATURVETENSKAP: NATURVETENSKAP; och Geovetenskap och ...; och Meteorologi och ...

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