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- Belanger-Chabot, Guillaume (author)
Ammonia-(Dinitramido)boranes: High-Energy-Density Materials.
- Article/chapterEnglish2015
Publisher, publication year, extent ...
- 2015-08-13
- Wiley,2015
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- LIBRIS-ID:oai:research.chalmers.se:2ea7a4bb-9eda-478a-9cbb-8e13b00805eb
- https://doi.org/10.1002/anie.201505684DOI
- https://research.chalmers.se/publication/249214URI
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- Language:English
- Summary in:English
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- Two ammonia-(dinitramido)boranes were synthesized by the reaction of dinitroamine with ammonia-borane. These compds. are the first reported examples of (dinitramido)boranes. Ammonia-mono(dinitramido)borane is a perfectly oxygen-balanced high-energy-d. material (HEDM) composed of an ammonia-BH2 fuel group and a strongly oxidizing dinitramido ligand. Although it is thermally not stable enough for practical applications, its predicted specific impulse as a solid rocket propellant would be 333 s. Its predicted performance as an explosive matches that of pentaerythtritol tetranitrate (PETN) and significantly exceeds that of trinitrotoluene (TNT). Its structure was established by X-ray crystallog. and vibrational and multinuclear NMR spectroscopy. Addnl., the over-oxidized ammoniabis(dinitramido)borane was detected by NMR spectroscopy. [on SciFinder(R)]
Subject headings and genre
- NATURVETENSKAP Kemi Oorganisk kemi hsv//swe
- NATURAL SCIENCES Chemical Sciences Inorganic Chemistry hsv//eng
- NATURVETENSKAP Kemi Materialkemi hsv//swe
- NATURAL SCIENCES Chemical Sciences Materials Chemistry hsv//eng
- NATURVETENSKAP Kemi Teoretisk kemi hsv//swe
- NATURAL SCIENCES Chemical Sciences Theoretical Chemistry hsv//eng
- dinitramido ligands
- energetic materials
- boranes
- quantum chemistry
- explosives
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- Rahm, Martin,1982 (author)
- Haiges, Ralf (author)
- Christe, Karl O. (author)
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- In:Angewandte Chemie - International Edition: Wiley54, s. 11730-117341433-78511521-3773
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