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  • Bilde, M.Århus Universitet,Aarhus University (author)

Saturation Vapor Pressures and Transition Enthalpies of Low-Volatility Organic Molecules of Atmospheric Relevance: From Dicarboxylic Acids to Complex Mixtures

  • Article/chapterEnglish2015

Publisher, publication year, extent ...

  • 2015-05-01
  • American Chemical Society (ACS),2015

Numbers

  • LIBRIS-ID:oai:research.chalmers.se:95f79dbf-ddf3-4e30-a986-93f086325972
  • https://research.chalmers.se/publication/219027URI
  • https://doi.org/10.1021/cr5005502DOI
  • https://lup.lub.lu.se/record/7612602URI
  • https://gup.ub.gu.se/publication/219027URI
  • https://urn.kb.se/resolve?urn=urn:nbn:se:su:diva-119064URI

Supplementary language notes

  • Language:English
  • Summary in:English

Part of subdatabase

Classification

  • Subject category:for swepub-publicationtype
  • Subject category:ref swepub-contenttype

Notes

  • There are a number of techniques that can be used that differ in terms of whether they fundamentally probe the equilibrium and the temperature range over which they can be applied. The series of homologous, straight-chain dicarboxylic acids have received much attention over the past decade given their atmospheric relevance, commercial availability, and low saturation vapor pressures, thus making them ideal test compounds. Uncertainties in the solid-state saturation vapor pressures obtained from individual methodologies are typically on the order of 50-100%, but the differences between saturation vapor pressures obtained with different methods are approximately 1-4 orders of magnitude, with the spread tending to increase as the saturation vapor pressure decreases. Some of the dicarboxylic acids can exist with multiple solid-state structures that have distinct saturation vapor pressures. Furthermore, the samples on which measurements are performed may actually exist as amorphous subcooled liquids rather than solid crystalline compounds, again with consequences for the measured saturation vapor pressures, since the subcooled liquid phase will have a higher saturation vapor pressure than the crystalline solid phase. Compounds with equilibrium vapor pressures in this range will exhibit the greatest sensitivities in terms of their gas to particle partitioning to uncertainties in their saturation vapor pressures, with consequent impacts on the ability of explicit and semiexplicit chemical models to simulate secondary organic aerosol formation.

Subject headings and genre

Added entries (persons, corporate bodies, meetings, titles ...)

  • Barsanti, K.Portland State University (author)
  • Booth, M.University of Manchester (author)
  • Cappa, C. D.University of California (author)
  • Donahue, N. M.Carnegie Mellon University (CMU) (author)
  • Emanuelsson, E. U.Århus Universitet,Aarhus University (author)
  • McFiggans, G.University of Manchester (author)
  • Krieger, U. K.Eidgenössische Technische Hochschule Zürich (ETH),Swiss Federal Institute of Technology in Zürich (ETH) (author)
  • Marcolli, C.Eidgenössische Technische Hochschule Zürich (ETH),Swiss Federal Institute of Technology in Zürich (ETH) (author)
  • Tropping, D.University of Manchester (author)
  • Ziemann, P.University of Colorado at Boulder (author)
  • Barley, M.University of Manchester (author)
  • Clegg, S.University of California (author)
  • Dennis-Smither, B.University of Bristol (author)
  • Hallquist, Mattias,1969Gothenburg University,Göteborgs universitet,Institutionen för kemi och molekylärbiologi,Department of Chemistry and Molecular Biology(Swepub:gu)xhamat (author)
  • Hallquist, Åsa M.IVL Svenska Miljöinstitutet AB,IVL Swedish Environmental Research Institute (author)
  • Khlystov, A.Desert Research Institute Reno, Division of Atmospheric Sciences (author)
  • Kulmala, M.Helsingin Yliopisto,University of Helsinki (author)
  • Mogensen, D.Helsingin Yliopisto,University of Helsinki (author)
  • Percival, C. J.University of Manchester (author)
  • Pope, F.University of Birmingham (author)
  • Pagels, JoakimLund University,Lunds universitet,Ergonomi och aerosolteknologi,Institutionen för designvetenskaper,Institutioner vid LTH,Lunds Tekniska Högskola,Ergonomics and Aerosol Technology,Department of Design Sciences,Departments at LTH,Faculty of Engineering, LTH(Swepub:lu)ie-jpa (author)
  • da Silva, MavrUniversidade do Porto,University of Porto (author)
  • Rosenoern, T.Köpenhamns universitet,University of Copenhagen (author)
  • Salo, Kent,1967Chalmers tekniska högskola,Chalmers University of Technology(Swepub:cth)kp01sake (author)
  • Soonsin, V. P.Eidgenössische Technische Hochschule Zürich (ETH),Swiss Federal Institute of Technology in Zürich (ETH),Chulalongkorn University (author)
  • Yli-Juuti, T.Itä-Suomen Yliopisto,University of Eastern Finland,Helsingin Yliopisto,University of Helsinki (author)
  • Prisle, N. L.Helsingin Yliopisto,University of Helsinki (author)
  • Pagels, J.Lunds universitet,Lund University (author)
  • Rarey, J.DDBST GmbH,Carl von Ossietzky Universität Oldenburg,The Carl von Ossietzky University of Oldenburg,University of KwaZulu-Natal (author)
  • Zardini, A. A.Europeiska kommissionens gemensamma forskningscentrum (JRC),Joint Research Centre (JRC), European Commission (author)
  • Riipinen, IlonaStockholms universitet,Institutionen för miljövetenskap och analytisk kemi(Swepub:su)iriip (author)
  • Århus UniversitetPortland State University (creator_code:org_t)

Related titles

  • In:Chemical Reviews: American Chemical Society (ACS)115:10, s. 4115-41560009-26651520-6890

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