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Sökning: WFRF:(Agostini Marco 1987) > Talyzin Aleksandr V. 1969 > Critical Role of Fu...

  • Sun, Jinhua,1987Chalmers tekniska högskola,Chalmers University of Technology,Department of Industrial and Materials Science, Chalmers University of Technology, Göteborg, Sweden (författare)

Critical Role of Functional Groups Containing N, S, and O on Graphene Surface for Stable and Fast Charging Li-S Batteries

  • Artikel/kapitelEngelska2021

Förlag, utgivningsår, omfång ...

  • 2021-03-14
  • Wiley,2021
  • electronicrdacarrier

Nummerbeteckningar

  • LIBRIS-ID:oai:research.chalmers.se:99360118-3d9f-4513-a4be-97618c1d2465
  • https://research.chalmers.se/publication/522876URI
  • https://research.chalmers.se/publication/522885URI
  • https://doi.org/10.1002/smll.202007242DOI
  • https://urn.kb.se/resolve?urn=urn:nbn:se:umu:diva-181840URI

Kompletterande språkuppgifter

  • Språk:engelska
  • Sammanfattning på:engelska

Ingår i deldatabas

Klassifikation

  • Ämneskategori:art swepub-publicationtype
  • Ämneskategori:ref swepub-contenttype

Anmärkningar

  • Lithium‐sulfur (Li‐S) batteries are considered one of the most promising energy storage technologies, possibly replacing the state‐of‐the‐art lithium‐ion (Li‐ion) batteries owing to their high energy density, low cost, and eco‐compatibility. However, the migration of high‐order lithium polysulfides (LiPs) to the lithium surface and the sluggish electrochemical kinetics pose challenges to their commercialization. The interactions between the cathode and LiPs can be enhanced by the doping of the carbon host with heteroatoms, however with relatively low doping content (<10%) in the bulk of the carbon, which can hardly interact with LiPs at the host surface. In this study, the grafting of versatile functional groups with designable properties (e.g., catalytic effects) directly on the surface of the carbon host is proposed to enhance interactions with LiPs. As model systems, benzene groups containing N/O and S/O atoms are vertically grafted and uniformly distributed on the surface of expanded reduced graphene oxide, fostering a stable interface between the cathode and LiPs. The combination of experiments and density functional theory calculations demonstrate improvements in chemical interactions between graphene and LiPs, with an enhancement in the electrochemical kinetics, power, and energy densities.

Ämnesord och genrebeteckningar

Biuppslag (personer, institutioner, konferenser, titlar ...)

  • Hwang, Jang YeonChonnam National University,Department of Materials Science and Engineering, Chonnam National University, 77 Yongbong-ro, Buk-gu, Gwangju, South Korea (författare)
  • Jankowski, Piotr,1990Wojskowa Akademia Techniczna im. Jarosława Dąbrowskiego w Warszawie - WAT,Military University of Technology in Warsaw,Danmarks Tekniske Universitet,Technical University of Denmark,Faculty of Chemistry, Warsaw University of Technology, Warsaw, Poland; Department of Energy Conversion and Storage, Technical University of Denmark, Kgs. Lyngby, Denmark(Swepub:cth)jpiotr (författare)
  • Xiao, LinhongUmeå universitet,Kemiska institutionen,Umeå University(Swepub:umu)lixi0004 (författare)
  • Sanchez Sanchez, Jaime,1990Chalmers tekniska högskola,Chalmers University of Technology,Department of Industrial and Materials Science, Chalmers University of Technology, Göteborg, Sweden(Swepub:cth)jaimes (författare)
  • Xia, Zhenyuan,1983Chalmers tekniska högskola,Chalmers University of Technology,Istituto per la Sintesi Organica e la Fotoreattività (ISOF-CNR),Institute for organic syntheses and photoreactivity (ISOF-CNR),Department of Industrial and Materials Science, Chalmers University of Technology, Göteborg, Sweden; Institute of Organic Synthesis and Photoreactivity (ISOF), CNR, via Gobetti 101, Bologna, Italy(Swepub:cth)zhenyuan (författare)
  • Lee, SuyeongChonnam National University,Department of Materials Science and Engineering, Chonnam National University, 77 Yongbong-ro, Buk-gu, Gwangju, South Korea (författare)
  • Talyzin, Aleksandr V.,1969-Umeå universitet,Institutionen för fysik,Umeå University(Swepub:umu)alta0001 (författare)
  • Matic, Aleksandar,1968Chalmers tekniska högskola,Chalmers University of Technology,Department of Physics, Chalmers University of Technology, Göteborg, Sweden(Swepub:cth)matic (författare)
  • Palermo, Vincenzo,1972Chalmers tekniska högskola,Chalmers University of Technology,Istituto per la Sintesi Organica e la Fotoreattività (ISOF-CNR),Institute for organic syntheses and photoreactivity (ISOF-CNR),Department of Industrial and Materials Science, Chalmers University of Technology, Göteborg, Sweden; Institute of Organic Synthesis and Photoreactivity (ISOF), CNR, via Gobetti 101, Bologna, Italy(Swepub:cth)palermo (författare)
  • Sun, Yang-KookHanyang University,Department of Energy Engineering, Hanyang University, Seoul, South Korea (författare)
  • Agostini, Marco,1987Chalmers tekniska högskola,Chalmers University of Technology,Department of Physics, Chalmers University of Technology, Göteborg, Sweden(Swepub:cth)agostini (författare)
  • Chalmers tekniska högskolaDepartment of Industrial and Materials Science, Chalmers University of Technology, Göteborg, Sweden (creator_code:org_t)

Sammanhörande titlar

  • Ingår i:Small: Wiley17:171613-68101613-6829

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