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Interfacial Approach toward Benzene-Bridged Polypyrrole Film–Based Micro-Supercapacitors with Ultrahigh Volumetric Power Density

Jiang, K. (author)
The Soft2D Lab, State Key Laboratory of Metal Matrix Composites, Shanghai Key Laboratory of Electrical Insulation and Thermal Ageing, School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai, 200240 China
Baburin, I. A. (author)
Center for Advancing Electronics Dresden & Department of Chemistry and Food Chemistry, Technische Universität Dresden, 01062 Dresden, Germany
Han, P. (author)
Max Planck Institute for Polymer Research, Ackermannweg 10, 55128 Mainz, Germany
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Yang, C. (author)
The Soft2D Lab, State Key Laboratory of Metal Matrix Composites, Shanghai Key Laboratory of Electrical Insulation and Thermal Ageing, School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai, 200240 China
Fu, X. (author)
Physics Department & Shanghai Key Laboratory of Magnetic Resonance, East China Normal University, North Zhongshan Road 3663, Shanghai, 200062 China
Yao, Y. (author)
Physics Department & Shanghai Key Laboratory of Magnetic Resonance, East China Normal University, North Zhongshan Road 3663, Shanghai, 200062 China
Li, Jiantong, 1980- (author)
KTH,Elektronik och inbyggda system
Cánovas, E. (author)
Max Planck Institute for Polymer Research, Ackermannweg 10, 55128 Mainz, Germany
Seifert, G. (author)
Center for Advancing Electronics Dresden & Department of Chemistry and Food Chemistry, Technische Universität Dresden, 01062 Dresden, Germany
Chen, J. (author)
The Soft2D Lab, State Key Laboratory of Metal Matrix Composites, Shanghai Key Laboratory of Electrical Insulation and Thermal Ageing, School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai, 200240 China
Bonn, M. (author)
Max Planck Institute for Polymer Research, Ackermannweg 10, 55128 Mainz, Germany
Feng, X. (author)
Center for Advancing Electronics Dresden & Department of Chemistry and Food Chemistry, Technische Universität Dresden, 01062 Dresden, Germany
Zhuang, X. (author)
The Soft2D Lab, State Key Laboratory of Metal Matrix Composites, Shanghai Key Laboratory of Electrical Insulation and Thermal Ageing, School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai, 200240 China
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 (creator_code:org_t)
2019-12-20
2020
English.
In: Advanced Functional Materials. - : Wiley. - 1616-301X .- 1616-3028. ; 30:7
Related links:
https://urn.kb.se/re...
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https://doi.org/10.1...
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  • Journal article (peer-reviewed)
Abstract Subject headings
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  • 2D soft nanomaterials are an emerging research field due to their versatile chemical structures, easily tunable properties, and broad application potential. In this study, a benzene‐bridged polypyrrole film with a large area, up to a few square centimeters, is synthesized through an interfacial polymerization approach. As‐prepared semiconductive films exhibit a bandgap of ≈2 eV and a carrier mobility of ≈1.5 cm2 V−1 s−1, inferred from time‐resolved terahertz spectroscopy. The samples are employed to fabricate in‐plane micro‐supercapacitors (MSCs) by laser scribing and exhibit an ultrahigh areal capacitance of 0.95 mF cm−2, using 1‐ethyl‐3‐methylimidazolium tetrafluoroborate ([EMIM][BF4]) as an electrolyte. Importantly, the maximum energy and power densities of the developed MSCs reach values up to 50.7 mWh cm−3 and 9.6 kW cm−3, respectively; the performance surpassing most of the 2D material‐based MSCs is reported to date.

Subject headings

TEKNIK OCH TEKNOLOGIER  -- Nanoteknik (hsv//swe)
ENGINEERING AND TECHNOLOGY  -- Nano-technology (hsv//eng)
NATURVETENSKAP  -- Kemi -- Materialkemi (hsv//swe)
NATURAL SCIENCES  -- Chemical Sciences -- Materials Chemistry (hsv//eng)

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ref (subject category)
art (subject category)

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