id:"swepub:oai:DiVA.org:kth-155466"
Sökning: id:"swepub:oai:DiVA.org:kth-155466" > Nickel Complex with...
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| Fältnamn | Indikatorer | Metadata |
|---|---|---|
| 000 | 02827naa a2200433 4500 | |
| 001 | oai:DiVA.org:kth-155466 | |
| 003 | SwePub | |
| 008 | 141106s2014 | |||||||||||000 ||eng| | |
| 024 | 7 | a https://urn.kb.se/resolve?urn=urn:nbn:se:kth:diva-1554662 URI |
| 024 | 7 | a https://doi.org/10.1002/cssc.2014023812 DOI |
| 040 | a (SwePub)kth | |
| 041 | a engb eng | |
| 042 | 9 SwePub | |
| 072 | 7 | a ref2 swepub-contenttype |
| 072 | 7 | a art2 swepub-publicationtype |
| 100 | 1 | a Yang, Yong4 aut |
| 245 | 1 0 | a Nickel Complex with Internal Bases as Efficient Molecular Catalyst for Photochemical H-2 Production |
| 264 | c 2014-09-01 | |
| 264 | 1 | b Wiley,c 2014 |
| 338 | a print2 rdacarrier | |
| 500 | a QC 20141113 | |
| 520 | a A Ni complex with internal bases that contain bipyridine-derived ligands, [Ni(L)(2)(H2O)(2)](BF4)(2) ([1](BF4)(2), L=2-(2-pyridyl)-1,8-naphthyridine), and a reference complex that bears analogous bipyridine-derived ligands but without an internal base, [Ni(L)(3)](BF4)(2) ([2](BF4)(2), L=2-(2-pyridyl)quinoline), were synthesized and characterized. The electrochemical properties of these complexes were studied in CH3CN, H2O, and a mixture of EtOH/H2O. The fluorescence spectroscopic studies suggest that both dynamic and the sphere-of-action static quenching exist in the fluorescein Fl(2-)/[1](2+) and Fl(2-)/[2](2+) systems. These noble-metal-free molecular systems were studied for photocatalytic H-2 generation. Under optimal conditions, the turnover number of H-2 evolution reaches 3230 based on [1](2+), whereas [2](2+) displays only approximately one third of the turnover of [1](2+). A plausible mechanism for the catalytic H-2 generation by [1](2+) is presented based on DFT calculations. | |
| 650 | 7 | a NATURVETENSKAPx Kemix Annan kemi0 (SwePub)104992 hsv//swe |
| 650 | 7 | a NATURAL SCIENCESx Chemical Sciencesx Other Chemistry Topics0 (SwePub)104992 hsv//eng |
| 653 | a density functional calculations | |
| 653 | a hydrogen | |
| 653 | a nickel | |
| 653 | a photochemistry | |
| 653 | a water splitting | |
| 700 | 1 | a Wang, Mei4 aut |
| 700 | 1 | a Xue, Liqinu KTH,Teoretisk kemi och biologi4 aut0 (Swepub:kth)u10eykwn |
| 700 | 1 | a Zhang, Fengbo4 aut |
| 700 | 1 | a Chen, Lin4 aut |
| 700 | 1 | a Ahlquist, Mårten S. G.u KTH,Teoretisk kemi och biologi4 aut0 (Swepub:kth)u1agoeae |
| 700 | 1 | a Sun, Lichengu KTH,Organisk kemi,State Key Laboratory of Fine Chemicals, DUT-KTH Education and Research Centre on Molecular Devices, Dalian University of Technology (DUT), China4 aut0 (Swepub:kth)u1umfd9h |
| 710 | 2 | a KTHb Teoretisk kemi och biologi4 org |
| 773 | 0 | t ChemSusChemd : Wileyg 7:10, s. 2889-2897q 7:10<2889-2897x 1864-5631x 1864-564X |
| 856 | 4 8 | u https://urn.kb.se/resolve?urn=urn:nbn:se:kth:diva-155466 |
| 856 | 4 8 | u https://doi.org/10.1002/cssc.201402381 |
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