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Layer-by-layer self...
Layer-by-layer self-assembly of pillared two-dimensional multilayers
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- Tian, Weiqian (author)
- KTH,Fiber- och polymerteknologi
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- Vahid Mohammadi, Armin (author)
- Auburn Univ, Dept Mech & Mat Engn, Auburn, AL 36849 USA.
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- Wang, Zhen (author)
- KTH,Fiber- och polymerteknologi
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- Ouyang, Liangqi (author)
- KTH,Fiber- och polymerteknologi
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- Beidaghi, Majid (author)
- Auburn Univ, Dept Mech & Mat Engn, Auburn, AL 36849 USA.
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- Hamedi, Mahiar M. (author)
- KTH,Fiber- och polymerteknologi
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(creator_code:org_t)
- 2019-06-11
- 2019
- English.
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In: Nature Communications. - : Nature Publishing Group. - 2041-1723. ; 10
- Related links:
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https://www.nature.c...
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https://urn.kb.se/re...
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https://doi.org/10.1...
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Abstract
Subject headings
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- We report Layer-by-Layer (LbL) self-assembly of pillared two-dimensional (2D) multilayers, from water, onto a wide range of substrates. This LbL method uses a small molecule, tris(2-aminoethyl) amine (TAEA), and a colloidal dispersion of Ti3C2Tx MXene to LbL self-assemble (MXene/TAEA)(n )multilayers, where n denotes the number of bilayers. Assembly with TAEA results in highly ordered (MXene/TAEA)(n) multilayers where the TAEA expands the interlayer spacing of MXene flakes by only similar to 1 angstrom and reinforces the interconnection between them. The TAEA-pillared MXene multilayers show the highest electronic conductivity of 7.3 x10(4) S m(-1) compared with all reported MXene multilayers fabricated by LbL technique. The (MXene/ TAEA)(n) multilayers could be used as electrodes for flexible all-solid-state supercapacitors delivering a high volumetric capacitance of 583 F cm(-3) and high energy and power densities of 3.0 Wh L-1 and 4400 W L-1, respectively. This strategy enables large-scale fabrication of highly conductive pillared MXene multilayers, and potentially fabrication of other 2D heterostructures.
Subject headings
- NATURVETENSKAP -- Kemi (hsv//swe)
- NATURAL SCIENCES -- Chemical Sciences (hsv//eng)
Publication and Content Type
- ref (subject category)
- art (subject category)
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