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Superlattice deformation in quantum dot films on flexible substrates via uniaxial strain

Heger, Julian E. (author)
Tech Univ Munich, Chair Funct Mat, TUM Sch Nat Sci, Dept Phys, James Franck Str 1, D-85748 Garching, Germany.
Chen, Wei (author)
Tech Univ Munich, Chair Funct Mat, TUM Sch Nat Sci, Dept Phys, James Franck Str 1, D-85748 Garching, Germany.;Shenzhen Technol Univ SZTU, Coll Engn Phys, Lantian Rd 3002, Shenzhen 518118, Peoples R China.
Zhong, Huaying (author)
Tech Univ Munich, Chair Funct Mat, TUM Sch Nat Sci, Dept Phys, James Franck Str 1, D-85748 Garching, Germany.
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Xiao, Tianxiao (author)
Tech Univ Munich, Chair Funct Mat, TUM Sch Nat Sci, Dept Phys, James Franck Str 1, D-85748 Garching, Germany.
Harder, Constantin (author)
Tech Univ Munich, Chair Funct Mat, TUM Sch Nat Sci, Dept Phys, James Franck Str 1, D-85748 Garching, Germany.;Deutsch Elektronen Synchrotron DESY, Notkestr 85, D-22607 Hamburg, Germany.
Apfelbeck, Fabian A. C. (author)
Tech Univ Munich, Chair Funct Mat, TUM Sch Nat Sci, Dept Phys, James Franck Str 1, D-85748 Garching, Germany.
Weinzierl, Alexander F. (author)
Tech Univ Munich, Chair Funct Mat, TUM Sch Nat Sci, Dept Phys, James Franck Str 1, D-85748 Garching, Germany.
Boldt, Regine (author)
Leibniz Inst Polymerforsch Dresden eV, Inst Polymerwerkstoffe, Hohe Str 6, D-01069 Dresden, Germany.
Schraa, Lucas (author)
Leibniz Inst Polymerforsch Dresden eV, Inst Polymerwerkstoffe, Hohe Str 6, D-01069 Dresden, Germany.
Euchler, Eric (author)
Leibniz Inst Polymerforsch Dresden eV, Inst Polymerwerkstoffe, Hohe Str 6, D-01069 Dresden, Germany.
Sambale, Anna K. (author)
Leibniz Inst Polymerforsch Dresden eV, Inst Polymerwerkstoffe, Hohe Str 6, D-01069 Dresden, Germany.
Schneider, Konrad (author)
Leibniz Inst Polymerforsch Dresden eV, Inst Polymerwerkstoffe, Hohe Str 6, D-01069 Dresden, Germany.
Schwartzkopf, Matthias (author)
Deutsch Elektronen Synchrotron DESY, Notkestr 85, D-22607 Hamburg, Germany.
Roth, Stephan V. (author)
KTH,Ytbehandlingsteknik,Deutsch Elektronen Synchrotron DESY, Notkestr 85, D-22607 Hamburg, Germany.
Mueller-Buschbaum, P. (author)
Tech Univ Munich, Chair Funct Mat, TUM Sch Nat Sci, Dept Phys, James Franck Str 1, D-85748 Garching, Germany.;Tech Univ Munich, Heinz Maier Leibnitz Zent MLZ, Lichtenbergstr 1, D-85748 Garching, Germany.
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Tech Univ Munich, Chair Funct Mat, TUM Sch Nat Sci, Dept Phys, James Franck Str 1, D-85748 Garching, Germany Tech Univ Munich, Chair Funct Mat, TUM Sch Nat Sci, Dept Phys, James Franck Str 1, D-85748 Garching, Germany.;Shenzhen Technol Univ SZTU, Coll Engn Phys, Lantian Rd 3002, Shenzhen 518118, Peoples R China. (creator_code:org_t)
2023
2023
English.
In: Nanoscale Horizons. - : Royal Society of Chemistry (RSC). - 2055-6764 .- 2055-6756. ; 8:3, s. 383-395
  • Journal article (peer-reviewed)
Abstract Subject headings
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  • The superlattice in a quantum dot (QD) film on a flexible substrate deformed by uniaxial strain shows a phase transition in unit cell symmetry. With increasing uniaxial strain, the QD superlattice unit cell changes from tetragonal to cubic to tetragonal phase as measured with in situ grazing-incidence small-angle X-ray scattering (GISAXS). The respective changes in the optoelectronic coupling are probed with photoluminescence (PL) measurements. The PL emission intensity follows the phase transition due to the resulting changing inter-dot distances. The changes in PL intensity accompany a redshift in the emission spectrum, which agrees with the Forster resonance energy transfer (FRET) theory. The results are essential for a fundamental understanding of the impact of strain on the performance of flexible devices based on QD films, such as wearable electronics and next-generation solar cells on flexible substrates.

Subject headings

NATURVETENSKAP  -- Fysik -- Den kondenserade materiens fysik (hsv//swe)
NATURAL SCIENCES  -- Physical Sciences -- Condensed Matter Physics (hsv//eng)

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