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Tunable CHA/AEI Zeolite Intergrowths with A Priori Biselective Organic Structure-Directing Agents : Controlling Enrichment and Implications for Selective Catalytic Reduction of NOx
- Bello-Jurado, Estefanía (author)
- Schwalbe-Koda, Daniel (author)
-
- Nero, Mathias (author)
- Stockholms universitet,Institutionen för material- och miljökemi (MMK)
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- Paris, Cecilia (author)
- Román-Leshkov, Yuriy (author)
- Corma, Avelino (author)
- Gómez-Bombarelli, Rafael (author)
- Moliner, Manuel (author)
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- (creator_code:org_t)
- 2022-05-19
- 2022
- English.
- In: Angewandte Chemie International Edition. - : Wiley. - 1433-7851 .- 1521-3773. ; 61:28
- Journal article (peer-reviewed)
Abstract
Subject headings
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- A novel ab initio methodology based on high-throughput simulations has permitted designing unique biselective organic structure-directing agents (OSDAs) that allow the efficient synthesis of CHA/AEI zeolite intergrowth materials with controlled phase compositions. Distinctive local crystallographic ordering of the CHA/AEI intergrowths was revealed at the nanoscale level using integrated differential phase contrast scanning transmission electron microscopy (iDPC STEM). These novel CHA/AEI materials have been tested for the selective catalytic reduction (SCR) of NOx, presenting an outstanding catalytic performance and hydrothermal stability, even surpassing the performance of the well-established commercial CHA-type catalyst. This methodology opens the possibility for synthetizing new zeolite intergrowths with more complex structures and unique catalytic properties.
Subject headings
- NATURVETENSKAP -- Kemi (hsv//swe)
- NATURAL SCIENCES -- Chemical Sciences (hsv//eng)
Keyword
- CHA/AEI intergrowths
- Biselective OSDAs
- Cu-containing zeolites
- SCR-NOx
- Machine Learning
Publication and Content Type
- ref (subject category)
- art (subject category)
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