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Core-hole localizat...
Core-hole localization and ultra-fast dissociation in SF6
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- Ekholm, V. (author)
- Uppsala University,Lund University,Lunds universitet,MAX IV-laboratoriet,MAX IV Laboratory
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- Chiuzbaian, G. S. (author)
- Sorbonne Univ, F-75005 Paris, France.;CNRS, LCPMR, F-75005 Paris, France.;Synchrotron SOLEIL, LOrme Merisiers, BP 48, F-91192 Gif Sur Yvette, France.,Lund Univ, MAX IV Lab, Box 118, SE-22100 Lund, Sweden.,Paris-Sorbonne University
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- S the, C. (author)
- Lund University,Lunds universitet,MAX IV-laboratoriet,MAX IV Laboratory
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- Nicolaou, A. (author)
- Synchrotron SOLEIL, LOrme Merisiers, BP 48, F-91192 Gif Sur Yvette, France.
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- Guarise, M. (author)
- Sorbonne Univ, F-75005 Paris, France.;CNRS, LCPMR, F-75005 Paris, France.;Ctr Nacl Pesquisa Energia & Mat CNPEM, BR-10000 Campinas, Brazil.,Brazilian Center For Research In Energy And Materials (CNPEM),Paris-Sorbonne University
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- Simon, M. (author)
- Sorbonne Univ, F-75005 Paris, France.;CNRS, LCPMR, F-75005 Paris, France.,Paris-Sorbonne University
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- Jaouen, N. (author)
- Synchrotron SOLEIL, LOrme Merisiers, BP 48, F-91192 Gif Sur Yvette, France.
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- Luning, J. (author)
- Sorbonne Univ, F-75005 Paris, France.;CNRS, LCPMR, F-75005 Paris, France.,Paris-Sorbonne University
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- Hague, C. F. (author)
- Sorbonne Univ, F-75005 Paris, France.;CNRS, LCPMR, F-75005 Paris, France.,Paris-Sorbonne University
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- Gel'mukhanov, Faris (author)
- KTH Royal Institute of Technology,KTH,Teoretisk kemi och biologi,Royal Inst Technol, Sch Biotechnol, Theoret Chem & Biol, S-10691 Stockholm, Sweden.;Siberian Fed Univ, Krasnoyarsk 660041, Russia.;Fed Res Ctr KSC SB RAS, Kirensky Inst Phys, Krasnoyarsk 660036, Russia.,Siberian Federal University,Kirensky Institute of Physics, Siberian Branch, Russian Academy of Sciences
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- Odelius, Michael (author)
- Stockholm University,Stockholms universitet,Fysikum,Stockholm Univ, AlbaNova Univ Ctr, Dept Phys, SE-10691 Stockholm, Sweden.
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- Björneholm, Olle (author)
- Uppsala University,Uppsala universitet,Molekyl- och kondenserade materiens fysik
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- Rubensson, Jan-Erik (author)
- Uppsala University,Uppsala universitet,Institutionen för fysik och astronomi
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(creator_code:org_t)
- 2020-07-24
- 2020
- English.
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In: Journal of Physics B. - : IOP Publishing. - 0953-4075 .- 1361-6455. ; 53:18
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Abstract
Subject headings
Close
- Resonant inelastic x-ray scattering spectra excited at the fluorine K resonances of SF(6)have been recorded. While a small but significant propensity for electronically parity-allowed transitions is found, the observation of parity-forbidden electronic transitions is attributed to vibronic coupling that breaks the global inversion symmetry of the electronic wavefunction and localizes the core hole. The dependence of the scattering cross section on the polarization of the incident radiation and the scattering angle is interpreted in terms of local pi/sigma symmetry around the S-F bond. This symmetry selectivity prevails during the dissociation that occurs during the scattering process.
Subject headings
- NATURVETENSKAP -- Fysik (hsv//swe)
- NATURAL SCIENCES -- Physical Sciences (hsv//eng)
- NATURVETENSKAP -- Fysik -- Atom- och molekylfysik och optik (hsv//swe)
- NATURAL SCIENCES -- Physical Sciences -- Atom and Molecular Physics and Optics (hsv//eng)
Keyword
- SF6
- resonant inelastic x-ray scattering
- symmetry selection rules
- ultrafast dynamics
- vibronic couplings
- resonant inelastic x-ray scattering
- SF
- symmetry selection rules
- ultrafast dynamics
- vibronic couplings
Publication and Content Type
- ref (subject category)
- art (subject category)
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To the university's database
- By the author/editor
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Ekholm, V.
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Chiuzbaian, G. S ...
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S the, C.
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Nicolaou, A.
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Guarise, M.
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Simon, M.
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show more...
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Jaouen, N.
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Luning, J.
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Hague, C. F.
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Gel'mukhanov, Fa ...
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Odelius, Michael
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Björneholm, Olle
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Rubensson, Jan-E ...
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show less...
- About the subject
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- NATURAL SCIENCES
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NATURAL SCIENCES
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and Physical Science ...
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- NATURAL SCIENCES
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NATURAL SCIENCES
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and Physical Science ...
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and Atom and Molecul ...
- Articles in the publication
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Journal of Physi ...
- By the university
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Royal Institute of Technology
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Stockholm University
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Uppsala University
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Lund University