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FältnamnIndikatorerMetadata
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001oai:DiVA.org:kth-290069
003SwePub
008210212s2020 | |||||||||||000 ||eng|
009oai:DiVA.org:uu-407449
009oai:lup.lub.lu.se:1ecf1f3d-2ed2-48cc-9e30-6a91fa52a822
0247 a https://urn.kb.se/resolve?urn=urn:nbn:se:kth:diva-2900692 URI
0247 a https://doi.org/10.1038/s41467-020-14468-w2 DOI
0247 a https://urn.kb.se/resolve?urn=urn:nbn:se:uu:diva-4074492 URI
0247 a https://lup.lub.lu.se/record/1ecf1f3d-2ed2-48cc-9e30-6a91fa52a8222 URI
040 a (SwePub)kthd (SwePub)uud (SwePub)lu
041 a engb eng
042 9 SwePub
072 7a ref2 swepub-contenttype
072 7a art2 swepub-publicationtype
1001 a Kunnus, Kristjanu Stanford Univ, PULSE Inst, SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA,Stanford Linear Accelerator Center (SLAC)4 aut
2451 0a Vibrational wavepacket dynamics in Fe carbene photosensitizer determined with femtosecond X-ray emission and scattering
264 c 2020-01-31
264 1b Springer Nature,c 2020
338 a electronic2 rdacarrier
500 a QC 20210215
520 a The non-equilibrium dynamics of electrons and nuclei govern the function of photoactive materials. Disentangling these dynamics remains a critical goal for understanding photoactive materials. Here we investigate the photoinduced dynamics of the [Fe(bmip)2]2+ photosensitizer, where bmip = 2,6-bis(3-methyl-imidazole-1-ylidine)-pyridine, with simultaneous femtosecond-resolution Fe Kα and Kβ X-ray emission spectroscopy (XES) and X-ray solution scattering (XSS). This measurement shows temporal oscillations in the XES and XSS difference signals with the same 278 fs period oscillation. These oscillations originate from an Fe-ligand stretching vibrational wavepacket on a triplet metal-centered (3MC) excited state surface. This 3MC state is populated with a 110 fs time constant by 40% of the excited molecules while the rest relax to a 3MLCT excited state. The sensitivity of the Kα XES to molecular structure results from a 0.7% average Fe-ligand bond length shift between the 1 s and 2p core-ionized states surfaces.
650 7a NATURVETENSKAPx Kemix Fysikalisk kemi0 (SwePub)104022 hsv//swe
650 7a NATURAL SCIENCESx Chemical Sciencesx Physical Chemistry0 (SwePub)104022 hsv//eng
650 7a NATURVETENSKAPx Fysikx Atom- och molekylfysik och optik0 (SwePub)103022 hsv//swe
650 7a NATURAL SCIENCESx Physical Sciencesx Atom and Molecular Physics and Optics0 (SwePub)103022 hsv//eng
7001 a Vacher, Morganeu Uppsala University,Uppsala universitet,Teoretisk kemi4 aut0 (Swepub:uu)morva594
7001 a Harlang, Tobias C.B.u Lund University,Lunds universitet,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Department of Physics,Departments at LTH,Faculty of Engineering, LTH,Technical University of Denmark4 aut0 (Swepub:lu)chem-tbh
7001 a Kjaer, Kasper S.u Stanford Univ, PULSE Inst, SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA;Lund Univ, Dept Chem Phys, POB 12, S-422100 Lund, Sweden;Tech Univ Denmark, Dept Phys, DK-2800 Lyngby, Denmark4 aut
7001 a Haldrup, Kristofferu Tech Univ Denmark, Dept Phys, DK-2800 Lyngby, Denmark,Technical University of Denmark4 aut
7001 a Biasin, Elisau Stanford Univ, PULSE Inst, SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA;Tech Univ Denmark, Dept Phys, DK-2800 Lyngby, Denmark,Stanford Linear Accelerator Center (SLAC),Technical University of Denmark4 aut
7001 a van Driel, Tim B.u SLAC Natl Accelerator Lab, LCLS, Menlo Pk, CA 94025 USA,Stanford Linear Accelerator Center (SLAC)4 aut
7001 a Papai, Matyasu Tech Univ Denmark, Dept Chem, Kemitorvet 207, DK-2800 Lyngby, Denmark,Technical University of Denmark4 aut
7001 a Chabera, Pavelu Lund University,Lunds universitet,NanoLund: Centre for Nanoscience,Annan verksamhet, LTH,Lunds Tekniska Högskola,Kemisk fysik,Enheten för fysikalisk och teoretisk kemi,Kemiska institutionen,Institutioner vid LTH,Other operations, LTH,Faculty of Engineering, LTH,Chemical Physics,Physical and theoretical chemistry,Department of Chemistry,Departments at LTH,Faculty of Engineering, LTH4 aut0 (Swepub:lu)chem-pcr
7001 a Liu, Yizhuu Lund University,Lunds universitet,Centrum för analys och syntes,Kemiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Kemisk fysik,Enheten för fysikalisk och teoretisk kemi,Centre for Analysis and Synthesis,Department of Chemistry,Departments at LTH,Faculty of Engineering, LTH,Chemical Physics,Physical and theoretical chemistry,Faculty of Engineering, LTH4 aut0 (Swepub:lu)orga-yhl
7001 a Tatsuno, Hideyukiu Lund University,Lunds universitet,Kemisk fysik,Enheten för fysikalisk och teoretisk kemi,Kemiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Chemical Physics,Physical and theoretical chemistry,Department of Chemistry,Departments at LTH,Faculty of Engineering, LTH4 aut0 (Swepub:lu)hi2364ta
7001 a Timm, Corneliau Lund Univ, Dept Chem Phys, POB 12, S-422100 Lund, Sweden,Lund University4 aut
7001 a Källman, Erik,c PhDu Uppsala University,Uppsala universitet,Teoretisk kemi4 aut0 (Swepub:uu)erika993
7001 a Delcey, Mickaëlu Uppsala University,Uppsala universitet,Teoretisk kemi4 aut0 (Swepub:lu)teok-mdl
7001 a Hartsock, Robert W.u Stanford Univ, PULSE Inst, SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA,Stanford Linear Accelerator Center (SLAC)4 aut
7001 a Reinhard, Marco E.u Stanford Univ, PULSE Inst, SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA,Stanford Linear Accelerator Center (SLAC)4 aut
7001 a Koroidov, Sergeyu Stanford Univ, PULSE Inst, SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA,Stanford Linear Accelerator Center (SLAC)4 aut
7001 a Laursen, Mads G.u Tech Univ Denmark, Dept Phys, DK-2800 Lyngby, Denmark,Technical University of Denmark4 aut
7001 a Hansen, Frederik B.u Tech Univ Denmark, Dept Phys, DK-2800 Lyngby, Denmark,Technical University of Denmark4 aut
7001 a Persson, Petteru Lund University,Lunds universitet,NanoLund: Centre for Nanoscience,Annan verksamhet, LTH,Lunds Tekniska Högskola,Beräkningskemi,Enheten för fysikalisk och teoretisk kemi,Kemiska institutionen,Institutioner vid LTH,Other operations, LTH,Faculty of Engineering, LTH,Computational Chemistry,Physical and theoretical chemistry,Department of Chemistry,Departments at LTH,Faculty of Engineering, LTH4 aut0 (Swepub:lu)chem-ppn
7001 a Christensen, Mortenu Tech Univ Denmark, Dept Phys, DK-2800 Lyngby, Denmark,Technical University of Denmark4 aut
7001 a Sandberg, Liseu Tech Univ Denmark, Dept Phys, DK-2800 Lyngby, Denmark;Univ Copenhagen, Niels Bohr Inst, Blegdamsvej 17, DK-2100 Copenhagen, Denmark,Technical University of Denmark,Niels Bohr Institute4 aut
7001 a Nemeth, Zoltanu Hungarian Acad Sci, Wigner Res Ctr Phys, POB 49, H-1525 Budapest, Hungary,Wigner Research Centre for Physics, Hungarian Academy of Sciences4 aut
7001 a Szemes, Dorottya Sarosineu Hungarian Acad Sci, Wigner Res Ctr Phys, POB 49, H-1525 Budapest, Hungary,Wigner Research Centre for Physics, Hungarian Academy of Sciences4 aut
7001 a Bajnoczi, Evau Hungarian Acad Sci, Wigner Res Ctr Phys, POB 49, H-1525 Budapest, Hungary,Wigner Research Centre for Physics, Hungarian Academy of Sciences4 aut
7001 a Alonso-Mori, Robertou SLAC Natl Accelerator Lab, LCLS, Menlo Pk, CA 94025 USA,Stanford Linear Accelerator Center (SLAC)4 aut
7001 a Glownia, James M.u SLAC Natl Accelerator Lab, LCLS, Menlo Pk, CA 94025 USA,Stanford Linear Accelerator Center (SLAC)4 aut
7001 a Nelson, Silkeu SLAC Natl Accelerator Lab, LCLS, Menlo Pk, CA 94025 USA,Stanford Linear Accelerator Center (SLAC)4 aut
7001 a Sikorski, Marcinu SLAC Natl Accelerator Lab, LCLS, Menlo Pk, CA 94025 USA,Stanford Linear Accelerator Center (SLAC)4 aut
7001 a Sokaras, Dimosthenisu SLAC Natl Accelerator Lab, SSRL, Menlo Pk, CA 94025 USA,Stanford Linear Accelerator Center (SLAC)4 aut
7001 a Lemke, Henrik T.u SLAC Natl Accelerator Lab, LCLS, Menlo Pk, CA 94025 USA,Stanford Linear Accelerator Center (SLAC)4 aut
7001 a Canton, Sophie E.u ELI HU Nonprofit Ltd, ELI ALPS, H-6720 Szeged, Hungary;DESY, Notkestr 85, D-22607 Hamburg, Germany,German Electron Synchrotron (DESY),ELI-HU Non-profit Ltd4 aut0 (Swepub:lu)chem-sca
7001 a Moller, Klaus B.u Tech Univ Denmark, Dept Chem, Kemitorvet 207, DK-2800 Lyngby, Denmark,Technical University of Denmark4 aut
7001 a Nielsen, Martin M.u Tech Univ Denmark, Dept Phys, DK-2800 Lyngby, Denmark,Technical University of Denmark4 aut
7001 a Vank, Gyorgyu Hungarian Acad Sci, Wigner Res Ctr Phys, POB 49, H-1525 Budapest, Hungary,Wigner Research Centre for Physics, Hungarian Academy of Sciences4 aut
7001 a Wärnmark, Kennethu Lund University,Lunds universitet,NanoLund: Centre for Nanoscience,Annan verksamhet, LTH,Lunds Tekniska Högskola,Centrum för analys och syntes,Kemiska institutionen,Institutioner vid LTH,Other operations, LTH,Faculty of Engineering, LTH,Centre for Analysis and Synthesis,Department of Chemistry,Departments at LTH,Faculty of Engineering, LTH4 aut0 (Swepub:lu)orgk1-kw
7001 a Sundström, Villyu Lund University,Lunds universitet,NanoLund: Centre for Nanoscience,Annan verksamhet, LTH,Lunds Tekniska Högskola,Kemisk fysik,Enheten för fysikalisk och teoretisk kemi,Kemiska institutionen,Institutioner vid LTH,Other operations, LTH,Faculty of Engineering, LTH,Chemical Physics,Physical and theoretical chemistry,Department of Chemistry,Departments at LTH,Faculty of Engineering, LTH4 aut0 (Swepub:lu)chph-vs
7001 a Persson, Petteru Lund Univ, Theoret Chem Div, POB 12422100, Lund, Sweden4 aut
7001 a Lundberg, Marcus,d 1974-u Uppsala University,Uppsala universitet,Teoretisk kemi4 aut0 (Swepub:uu)marlu250
7001 a Uhlig, Jensu Lund University,Lunds universitet,NanoLund: Centre for Nanoscience,Annan verksamhet, LTH,Lunds Tekniska Högskola,Kemisk fysik,Enheten för fysikalisk och teoretisk kemi,Kemiska institutionen,Institutioner vid LTH,Other operations, LTH,Faculty of Engineering, LTH,Chemical Physics,Physical and theoretical chemistry,Department of Chemistry,Departments at LTH,Faculty of Engineering, LTH4 aut0 (Swepub:lu)chem-jnu
7001 a Gaffney, Kelly J.u Stanford Univ, PULSE Inst, SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA,Stanford Linear Accelerator Center (SLAC)4 aut
7001 a Kjær, Kasper S.u Lund University,Lunds universitet,Kemisk fysik,Enheten för fysikalisk och teoretisk kemi,Kemiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Chemical Physics,Physical and theoretical chemistry,Department of Chemistry,Departments at LTH,Faculty of Engineering, LTH,Stanford Linear Accelerator Center (SLAC),Technical University of Denmark4 aut0 (Swepub:lu)chem-kkr
7102 a Stanford Univ, PULSE Inst, SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USAb Stanford Linear Accelerator Center (SLAC)4 org
7730 t Nature Communicationsd : Springer Natureg 11:1q 11:1x 2041-1723
8564 u https://doi.org/10.1038/s41467-020-14468-wy Fulltext
8564 u https://kth.diva-portal.org/smash/get/diva2:1527953/FULLTEXT01.pdfx primaryx Raw objecty fulltext:print
8564 u https://www.nature.com/articles/s41467-020-14468-w.pdf
8564 u https://uu.diva-portal.org/smash/get/diva2:1416740/FULLTEXT01.pdfx primaryx Raw objecty fulltext:print
8564 u http://dx.doi.org/10.1038/s41467-020-14468-wx freey FULLTEXT
8564 8u https://urn.kb.se/resolve?urn=urn:nbn:se:kth:diva-290069
8564 8u https://doi.org/10.1038/s41467-020-14468-w
8564 8u https://urn.kb.se/resolve?urn=urn:nbn:se:uu:diva-407449
8564 8u https://lup.lub.lu.se/record/1ecf1f3d-2ed2-48cc-9e30-6a91fa52a822

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