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Over 16% efficiency...
Over 16% efficiency organic photovoltaic cells enabled by a chlorinated acceptor with increased open-circuit voltages
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- Cui, Yong (author)
- Chinese Acad Sci, Peoples R China; Univ Chinese Acad Sci, Peoples R China
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- Yao, Huifeng (author)
- Chinese Acad Sci, Peoples R China
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- Zhang, Jianqi (author)
- Natl Ctr Nanosci and Technol, Peoples R China
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- Zhang, Tao (author)
- Chinese Acad Sci, Peoples R China
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- Wang, Yuming (author)
- Linköpings universitet,Biomolekylär och Organisk Elektronik,Tekniska fakulteten
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- Hong, Ling (author)
- Chinese Acad Sci, Peoples R China; Univ Chinese Acad Sci, Peoples R China
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- Xian, Kaihu (author)
- Chinese Acad Sci, Peoples R China; Univ Chinese Acad Sci, Peoples R China
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- Xu, Bowei (author)
- Chinese Acad Sci, Peoples R China
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- Zhang, Shaoqing (author)
- Chinese Acad Sci, Peoples R China; Univ Sci and Technol Beijing, Peoples R China
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- Peng, Jing (author)
- Organtec Ltd, Peoples R China
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- Wei, Zhixiang (author)
- Natl Ctr Nanosci and Technol, Peoples R China
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- Gao, Feng (author)
- Linköpings universitet,Biomolekylär och Organisk Elektronik,Tekniska fakulteten
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- Hou, Jianhui (author)
- Chinese Acad Sci, Peoples R China; Univ Chinese Acad Sci, Peoples R China
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(creator_code:org_t)
- 2019-06-07
- 2019
- English.
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In: Nature Communications. - : NATURE PUBLISHING GROUP. - 2041-1723. ; 10
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Abstract
Subject headings
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- Broadening the optical absorption of organic photovoltaic (OPV) materials by enhancing the intramolecular push-pull effect is a general and effective method to improve the power conversion efficiencies of OPV cells. However, in terms of the electron acceptors, the most common molecular design strategy of halogenation usually results in down-shifted molecular energy levels, thereby leading to decreased open-circuit voltages in the devices. Herein, we report a chlorinated non-fullerene acceptor, which exhibits an extended optical absorption and meanwhile displays a higher voltage than its fluorinated counterpart in the devices. This unexpected phenomenon can be ascribed to the reduced non-radiative energy loss (0.206 eV). Due to the simultaneously improved short-circuit current density and open-circuit voltage, a high efficiency of 16.5% is achieved. This study demonstrates that finely tuning the OPV materials to reduce the bandgap-voltage offset has great potential for boosting the efficiency.
Subject headings
- NATURVETENSKAP -- Fysik -- Annan fysik (hsv//swe)
- NATURAL SCIENCES -- Physical Sciences -- Other Physics Topics (hsv//eng)
Publication and Content Type
- ref (subject category)
- art (subject category)
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- By the author/editor
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Cui, Yong
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Yao, Huifeng
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Zhang, Jianqi
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Zhang, Tao
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Wang, Yuming
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Hong, Ling
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show more...
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Xian, Kaihu
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Xu, Bowei
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Zhang, Shaoqing
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Peng, Jing
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Wei, Zhixiang
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Gao, Feng
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Hou, Jianhui
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show less...
- About the subject
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- NATURAL SCIENCES
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NATURAL SCIENCES
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and Physical Science ...
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and Other Physics To ...
- Articles in the publication
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Nature Communica ...
- By the university
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Linköping University