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Two colour pump-probe study and internal energy dependence of Rydberg state excitation
- Boyle, Mark (author)
-
- Hedén, Martin, 1976 (author)
- Gothenburg University,Göteborgs universitet,Institutionen för fysik (GU),Department of Physics (GU)
- Schulz, C.P. (author)
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- Hertel, Ingolf, 1941 (author)
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- (creator_code:org_t)
- 2004
- 2004
- English.
- In: Physical Review A. - 1050-2947. ; 70
- Journal article (peer-reviewed)
Abstract
Subject headings
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- Excitation of Rydberg states in isolated C60 is studied by time-resolved photoelectron spectroscopy in a femtosecond two-color pump-probe experiment. The relaxation time for electron-electron interaction is determined to be approximately 100 fs with the t1g(LUMO + 1) orbital being considered to define the doorway state in a nonadiabatic multielectron excitation process. The internal energy stored in vibrational modes of the C60 at 770 K is found to support the excitation process very efficiently while in "cold" C60 (80 K), no significant Rydberg population is detected.
Subject headings
- NATURVETENSKAP -- Fysik -- Atom- och molekylfysik och optik (hsv//swe)
- NATURAL SCIENCES -- Physical Sciences -- Atom and Molecular Physics and Optics (hsv//eng)
Keyword
- fullerene spectroscopy
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- ref (subject category)
- art (subject category)
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