Sökning: onr:"swepub:oai:research.chalmers.se:2b60d556-d1d3-4eb3-be83-91c78db66b57" > Influence of the pl...
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000 | 03197naa a2200433 4500 | |
001 | oai:research.chalmers.se:2b60d556-d1d3-4eb3-be83-91c78db66b57 | |
003 | SwePub | |
008 | 171007s1998 | |||||||||||000 ||eng| | |
024 | 7 | a https://research.chalmers.se/publication/1548072 URI |
040 | a (SwePub)cth | |
041 | a engb eng | |
042 | 9 SwePub | |
072 | 7 | a art2 swepub-publicationtype |
072 | 7 | a ref2 swepub-contenttype |
100 | 1 | a Acke, Filip,d 1968u Chalmers tekniska högskola,Chalmers University of Technology4 aut |
245 | 1 0 | a Influence of the platinum-support interaction on the direct reduction of NOx under lean conditions |
264 | 1 | c 1998 |
520 | a Catalysts containing Pt supported on SiC, Al2O3 and ZSM-5 were prepared and studied for NOx reduction by C3H6 in Oz excess under transient (temperature ramps) and steady-state conditions. The maximum NOx reduction activity in the heating ramp experiments was similar for Pt/SiC and Pt/ZSM-5, while Pt/Al2O3 showed higher maximum activity. Both N-2 and N2O formation was observed for all catalysts, although the respective amounts varied with the investigated system. Highest Nz selectivity was observed for Pt/Al2O3. When the NOx reduction activity was studied under steady-state conditions the activity of Pt/Al2O3 decreased substantially (mainly due to a loss in N-2 production). Pt/ZSM-5 became somewhat more selective towards Na production whereas the activity and selectivity of Pt/SiC remained at about the same values as far the heating ramp experiments. Adsorbed species on the surface of the different catalysts were investigated using in-situ FTIR in order to obtain information about the reaction mechanisms. The adsorption of species on Pt/SiC was negligible, while a number of absorption bands were observed for Pt/Al2O3 (N and C containing species, and -NCO) and Pt/ZSM-5 (HC). | |
650 | 7 | a TEKNIK OCH TEKNOLOGIERx Kemiteknik0 (SwePub)2042 hsv//swe |
650 | 7 | a ENGINEERING AND TECHNOLOGYx Chemical Engineering0 (SwePub)2042 hsv//eng |
653 | a HYDROCARBONS | |
653 | a SELECTIVE CATALYTIC REDUCTION | |
653 | a PROPYLENE | |
653 | a EXCESS OXYGEN | |
653 | a ADSORPTION | |
653 | a SPECTROSCOPY | |
653 | a NITRIC-OXIDE | |
653 | a CO | |
653 | a RH/AL2O3 | |
653 | a STABILITY | |
700 | 1 | a Westerberg, Björn,d 1962u Chalmers tekniska högskola,Chalmers University of Technology4 aut |
700 | 1 | a Eriksson, Lars,d 1965u Chalmers tekniska högskola,Chalmers University of Technology4 aut |
700 | 1 | a Johansson, Stefan,d 1967u Chalmers tekniska högskola,Chalmers University of Technology4 aut |
700 | 1 | a Skoglundh, Magnus,d 1965u Chalmers tekniska högskola,Chalmers University of Technology4 aut0 (Swepub:cth)skoglund |
700 | 1 | a Fridell, Erik,d 1963u Chalmers tekniska högskola,Chalmers University of Technology4 aut0 (Swepub:cth)fridell |
700 | 1 | a Smedler, Gudmund,d 1956u Chalmers tekniska högskola,Chalmers University of Technology4 aut |
710 | 2 | a Chalmers tekniska högskola4 org |
773 | 0 | t Studies in Surface Science and Catalysisg 116, s. 285-294q 116<285-294x 0167-2991 |
856 | 4 8 | u https://research.chalmers.se/publication/154807 |
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