Sökning: L773:0939 5075 OR L773:1865 7125 > Biocatalysis for te...
Fältnamn | Indikatorer | Metadata |
---|---|---|
000 | 03118naa a2200433 4500 | |
001 | oai:DiVA.org:kth-246249 | |
003 | SwePub | |
008 | 190402s2019 | |||||||||||000 ||eng| | |
024 | 7 | a https://urn.kb.se/resolve?urn=urn:nbn:se:kth:diva-2462492 URI |
024 | 7 | a https://doi.org/10.1515/znc-2018-01992 DOI |
040 | a (SwePub)kth | |
041 | a engb eng | |
042 | 9 SwePub | |
072 | 7 | a ref2 swepub-contenttype |
072 | 7 | a art2 swepub-publicationtype |
100 | 1 | a Farhat, Wissamu KTH,Ytbehandlingsteknik,Science for Life Laboratory, SciLifeLab4 aut0 (Swepub:kth)u1695ok5 |
245 | 1 0 | a Biocatalysis for terpene-based polymers |
264 | c 2019-02-21 | |
264 | 1 | b WALTER DE GRUYTER GMBH,c 2019 |
338 | a print2 rdacarrier | |
500 | a QC 20190402 | |
520 | a Accelerated generation of bio-based materials is vital to replace current synthetic polymers obtained from petroleum with more sustainable options. However, many building blocks available from renewable resources mainly contain unreactive carbon-carbon bonds, which obstructs their efficient polymerization. Herein, we highlight the potential of applying biocatalysis to afford tailored functionalization of the inert carbocyclic core of multicyclic terpenes toward advanced materials. As a showcase, we unlock the inherent monomer reactivity of norcamphor, a bicyclic ketone used as a monoterpene model system in this study, to afford polyesters with unprecedented backbones. The efficiencies of the chemical and enzymatic Baeyer-Villiger transformation in generating key lactone intermediates are compared. The concepts discussed herein are widely applicable for the valorization of terpenes and other cyclic building blocks using chemoenzymatic strategies. | |
650 | 7 | a NATURVETENSKAPx Kemix Polymerkemi0 (SwePub)104062 hsv//swe |
650 | 7 | a NATURAL SCIENCESx Chemical Sciencesx Polymer Chemistry0 (SwePub)104062 hsv//eng |
653 | a biocatalysis | |
653 | a biopolymers | |
653 | a oxidoreductases | |
653 | a polyesters | |
653 | a terpenes | |
700 | 1 | a Stamm, Arneu KTH,Science for Life Laboratory, SciLifeLab,Ytbehandlingsteknik4 aut0 (Swepub:kth)u1m0o5w8 |
700 | 1 | a Robert-Monpate, Maximeu KTH,Ytbehandlingsteknik,Science for Life Laboratory, SciLifeLab,Ecole Super Chim Organ & Minerale, 1 Allee Reseau Jean Marie Buckmaster, F-60200 Compiegne, France4 aut0 (Swepub:kth)u1i93i9o |
700 | 1 | a Biundo, Antoninou KTH,Science for Life Laboratory, SciLifeLab,Ytbehandlingsteknik4 aut0 (Swepub:kth)u1l1ee04 |
700 | 1 | a Syrén, Per-Olofu KTH,Science for Life Laboratory, SciLifeLab,Ytbehandlingsteknik4 aut0 (Swepub:kth)u1ewlo1g |
710 | 2 | a KTHb Ytbehandlingsteknik4 org |
773 | 0 | t Zeitschrift für Naturforschung C - A Journal of Biosciencesd : WALTER DE GRUYTER GMBHg 74:3-4, s. 90-99q 74:3-4<90-99x 0939-5075x 1865-7125 |
856 | 4 | u https://doi.org/10.1515/znc-2018-0199y Fulltext |
856 | 4 | u https://www.degruyter.com/downloadpdf/journals/znc/74/3-4/article-p91.pdf |
856 | 4 8 | u https://urn.kb.se/resolve?urn=urn:nbn:se:kth:diva-246249 |
856 | 4 8 | u https://doi.org/10.1515/znc-2018-0199 |
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