The presence, emission and partitioning behavior of polychlorinated biphenyls in waste, leachate and aerosols from Norwegian waste-handling facilities

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Fältnamn	Indikatorer	Metadata
000		03767naa a2200469 4500
001		oai:DiVA.org:umu-169377
003		SwePub
008		200406s2020 \| \|\|\|\|\|\|\|\|\|\|\|000 \|\|eng\|
024	7	a https://urn.kb.se/resolve?urn=urn:nbn:se:umu:diva-1693772 URI
024	7	a https://doi.org/10.1016/j.scitotenv.2020.1368242 DOI
040		a (SwePub)umu
041		a engb eng
042		9 SwePub
072	7	a ref2 swepub-contenttype
072	7	a art2 swepub-publicationtype
100	1	a Arp, Hans Peter H.4 aut
245	1 0	a The presence, emission and partitioning behavior of polychlorinated biphenyls in waste, leachate and aerosols from Norwegian waste-handling facilities
264	1	b ELSEVIER,c 2020
338		a electronic2 rdacarrier
520		a Even though production and open use of polychlorinated biphenyls (PCBs) have been phased out in Western industrialised countries since the 1980s, PCBs were still present in waste collected from different waste handling facilities in Norway in 2013. Sums of seven indicator-PCBs (I-PCB7:PCB-28, -52, -101, -118, -138, -153 and -180) were highest in plastic waste (3700 +/- 1800 mu g/kg, n=15), waste electrical and electronic equipment (WEEE) (1300 +/- 400 mu g/kg, n=12) and fine vehicle fluff (1800 = 1400 mu g/kg, n=4) and lowest in glass waste, combustibles, bottom ash and fly ash (0.3 to 65 mu g/kg). Concentrations in leachate water varied from 1.7 to 2900 ng/L, with higher concentrations found at vehicle and WEEE handling facilities. Particles in leachate water exhibited similar PCB sorption properties as solid waste collected on site, with waste-water partitioning coefficients ranging from 10(5)to 10(7) .I-PCB7 in air samples collected at the sites were mostly in the gas phase (100-24000 pg/m(3)), compared to those associated with particles (9-1900 pg/m(3)). In contrast, brominated flame retardants (BFRs) in the same samples were predominantly found associated with particles (e.g. sum of 10 brominated diethyl ethers, Sigma BDE10, associated with particles 77-194,000 pg/m(3)) compared to the gas phase (Sigma DE10 6-473 pg/m(3)). Measured gas-phase I-PCB7 concentrations are less than predicted, assuming waste-air partitioning in equilibrium with predominant waste on site. However, the gas-particle partitioning behavior of PCBs and BFRs could be predicted using an established partitioning model for ambient aerosols. PCB emissions from Norwegian waste handling facilities occurred primarily in the form of atmospheric vapor or leachate particles.
650	7	a NATURVETENSKAPx Geovetenskap och miljövetenskapx Miljövetenskap0 (SwePub)105022 hsv//swe
650	7	a NATURAL SCIENCESx Earth and Related Environmental Sciencesx Environmental Sciences0 (SwePub)105022 hsv//eng
653		a Waste
653		a Recycling
653		a Leachate
653		a Gas-particle
653		a Emissions
653		a WEEE
653		a Plastic
700	1	a Morin, Nicolas A. O.4 aut
700	1	a Andersson, Patrik L.u Umeå universitet,Kemiska institutionen4 aut0 (Swepub:umu)paan0001
700	1	a Hale, Sarah E.4 aut
700	1	a Wania, Frank4 aut
700	1	a Breivik, Knut4 aut
700	1	a Breedveld, Gijs D.4 aut
710	2	a Umeå universitetb Kemiska institutionen4 org
773	0	t Science of the Total Environmentd : ELSEVIERg 715, s. 1-12q 715<1-12x 0048-9697x 1879-1026
856	4	u https://doi.org/10.1016/j.scitotenv.2020.136824y Fulltext
856	4	u https://umu.diva-portal.org/smash/get/diva2:1421803/FULLTEXT01.pdfx primaryx Raw objecty fulltext:print
856	4	u https://doi.org/10.1016/j.scitotenv.2020.136824
856	4 8	u https://urn.kb.se/resolve?urn=urn:nbn:se:umu:diva-169377
856	4 8	u https://doi.org/10.1016/j.scitotenv.2020.136824

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