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Femtosecond interatomic Coulombic decay in free neon clusters: Large lifetime differences between surface and bulk
- Ohrwall, G (author)
-
- Tchaplyguine, Maxim (author)
- Lund University,Lunds universitet,MAX IV-laboratoriet,MAX IV Laboratory
- Lundwall, M (author)
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- Feifel, R (author)
- Bergersen, H (author)
- Rander, T (author)
- Lindblad, A (author)
- Barth, S (author)
- Marburger, S (author)
- Hergenhahn, U (author)
- Svensson, S (author)
- Bjorneholm, O (author)
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- (creator_code:org_t)
- 2004
- 2004
- English.
- In: Physical Review Letters. - 1079-7114. ; 93:17
- Journal article (peer-reviewed)
Abstract
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- A quantitative determination of 2s vacancy lifetimes in surface and bulk atoms of free Ne clusters has been made. While for free atoms the 2s inner-valence hole has a ps lifetime, it reduces to 6+/-1 fs for cluster bulk atoms. For surface atoms, the lifetime is on average longer than 30 fs. The lifetime estimate was obtained from fits of high-resolution photoelectron spectra of Ne clusters. The shortening of the lifetime is attributed to the coordination dependent interatomic Coulombic decay, which is extremely sensitive to internuclear distances.
Subject headings
- NATURVETENSKAP -- Fysik (hsv//swe)
- NATURAL SCIENCES -- Physical Sciences (hsv//eng)
- NATURVETENSKAP -- Fysik -- Atom- och molekylfysik och optik (hsv//swe)
- NATURAL SCIENCES -- Physical Sciences -- Atom and Molecular Physics and Optics (hsv//eng)
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- ref (subject category)
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- Lindblad, A
- Schulz, Joachim
- Peredkov, Sergey
- Barth, S
- Marburger, S
- Hergenhahn, U
- Svensson, S
- Bjorneholm, O
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