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Defect-Passivation Using Organic Dyes for Enhanced Efficiency and Stability of Perovskite Solar Cells

Xiong, Shaobing (author)
East China Normal Univ, Peoples R China
Song, Jingnan (author)
Shanghai Jiao Tong Univ, Peoples R China
Yang, Jianming (author)
East China Normal Univ, Peoples R China
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Xu, Jinqiu (author)
Shanghai Jiao Tong Univ, Peoples R China
Zhang, Ming (author)
Shanghai Jiao Tong Univ, Peoples R China
Ma, Ruru (author)
East China Normal Univ, Peoples R China
Li, Danqin (author)
East China Normal Univ, Peoples R China
Liu, Xianjie (author)
Linköpings universitet,Laboratoriet för organisk elektronik,Tekniska fakulteten
Liu, Feng (author)
Shanghai Jiao Tong Univ, Peoples R China
Duan, Chungang (author)
East China Normal Univ, Peoples R China; Shanxi Univ, Peoples R China
Fahlman, Mats (author)
Linköpings universitet,Laboratoriet för organisk elektronik,Tekniska fakulteten
Bao, Qinye (author)
Linköpings universitet,Laboratoriet för organisk elektronik,Tekniska fakulteten,East China Normal Univ, Peoples R China; Shanxi Univ, Peoples R China
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 (creator_code:org_t)
2020-01-29
2020
English.
In: Solar RRL. - : WILEY-V C H VERLAG GMBH. - 2367-198X. ; 4:5
  • Journal article (peer-reviewed)
Abstract Subject headings
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  • Perovskite solar cells are a highly competitive candidate for next-generation photovoltaic technology. Defects in the perovskite grain boundaries and on the film surfaces however have significant impacts on both the device efficiency and environmental stability. Herein, a strategy using organic dyes as additives to passivate the defect states and produce more n-type perovskite films, thereby improving charge transport and decreasing charge recombination, is reported. Based on this strategy, the power conversion efficiency of the perovskite solar cell is significantly increased from 18.13% to 20.18% with a negligible hysteresis. Furthermore, the rich hydrogen bonds and carbonyl structures in the organic dye can significantly enhance device stability both in terms of humidity and thermal stress. The results present a promising pathway using abundant and colorful organic dyes as additives to achieve high-performance perovskite solar cells.

Subject headings

NATURVETENSKAP  -- Kemi -- Materialkemi (hsv//swe)
NATURAL SCIENCES  -- Chemical Sciences -- Materials Chemistry (hsv//eng)

Keyword

defect-passivation; efficiency; organic dyes; perovskite solar cells; stability

Publication and Content Type

ref (subject category)
art (subject category)

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