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Multicomponent new ...
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Lehtipalo, Katrianne
(author)
Multicomponent new particle formation from sulfuric acid, ammonia, and biogenic vapors
- Article/chapterEnglish2018
Publisher, publication year, extent ...
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American Association for the Advancement of Science (AAAS),2018
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printrdacarrier
Numbers
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LIBRIS-ID:oai:DiVA.org:su-165730
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https://urn.kb.se/resolve?urn=urn:nbn:se:su:diva-165730URI
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https://doi.org/10.1126/sciadv.aau5363DOI
Supplementary language notes
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Language:English
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Summary in:English
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Classification
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Subject category:ref swepub-contenttype
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Subject category:art swepub-publicationtype
Notes
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A major fraction of atmospheric aerosol particles, which affect both air quality and climate, form from gaseous precursors in the atmosphere. Highly oxygenated organic molecules (HOMs), formed by oxidation of biogenic volatile organic compounds, are known to participate in particle formation and growth. However, it is not well understood how they interact with atmospheric pollutants, such as nitrogen oxides (NOx) and sulfur oxides (SOx) from fossil fuel combustion, as well as ammonia (NH3) from livestock and fertilizers. Here, we show how NOx suppresses particle formation, while HOMs, sulfuric acid, and NH3 have a synergistic enhancing effect on particle formation. We postulate a novel mechanism, involving HOMs, sulfuric acid, and ammonia, which is able to closely reproduce observations of particle formation and growth in daytime boreal forest and similar environments. The findings elucidate the complex interactions between biogenic and anthropogenic vapors in the atmospheric aerosol system.
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Yan, Chao
(author)
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Dada, Lubna
(author)
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Bianchi, Federico
(author)
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Xiao, Mao
(author)
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Wagner, Robert
(author)
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Stolzenburg, Dominik
(author)
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Ahonen, Lauri R.
(author)
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Amorim, Antonio
(author)
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Baccarini, Andrea
(author)
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Bauer, Paulus S.
(author)
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Baumgartner, Bernhard
(author)
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Bergen, Anton
(author)
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Bernhammer, Anne-Kathrin
(author)
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Breitenlechner, Martin
(author)
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Brilke, Sophia
(author)
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Buchholz, Angela
(author)
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Mazon, Stephany Buenrostro
(author)
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Chen, Dexian
(author)
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Chen, Xuemeng
(author)
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Dias, Antonio
(author)
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Dommen, Josef
(author)
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Draper, Danielle C.
(author)
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Duplissy, Jonathan
(author)
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Ehn, Mikael
(author)
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Finkenzeller, Henning
(author)
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Fischer, Lukas
(author)
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Frege, Carla
(author)
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Fuchs, Claudia
(author)
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Garmash, Olga
(author)
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Gordon, Hamish
(author)
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Hakala, Jani
(author)
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He, Xucheng
(author)
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Heikkinen, Liine
(author)
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Heinritzi, Martin
(author)
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Helm, Johanna C.
(author)
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Hofbauer, Victoria
(author)
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Hoyle, Christopher R.
(author)
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Jokinen, Tuija
(author)
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Kangasluoma, Juha
(author)
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Kerminen, Veli-Matti
(author)
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Kim, Changhyuk
(author)
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Kirkby, Jasper
(author)
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Kontkanen, JenniStockholms universitet,Institutionen för miljövetenskap och analytisk kemi,University of Helsinki, Finland
(author)
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Kuerten, Andreas
(author)
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Lawler, Michael J.
(author)
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Mai, Huajun
(author)
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Mathot, Serge
(author)
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Mauldin, Roy L.
(author)
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Molteni, Ugo
(author)
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Nichman, Leonid
(author)
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Nie, Wei
(author)
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Nieminen, Tuomo
(author)
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Ojdanic, Andrea
(author)
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Onnela, Antti
(author)
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Passananti, Monica
(author)
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Petaja, Tuukka
(author)
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Piel, Felix
(author)
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Pospisilova, Veronika
(author)
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Quelever, Lauriane L. J.
(author)
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Rissanen, Matti P.
(author)
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Rose, Clemence
(author)
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Sarnela, Nina
(author)
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Schallhart, Simon
(author)
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Schuchmann, Simone
(author)
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Sengupta, Kamalika
(author)
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Simon, Mario
(author)
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Sipila, Mikko
(author)
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Tauber, Christian
(author)
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Tome, Antonio
(author)
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Trostl, Jasmin
(author)
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Vaisanen, Olli
(author)
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Vogel, Alexander L.
(author)
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Volkamer, Rainer
(author)
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Wagner, Andrea C.
(author)
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Wang, Mingyi
(author)
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Weitz, Lena
(author)
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Wimmer, Daniela
(author)
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Ye, Penglin
(author)
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Ylisirnio, Arttu
(author)
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Zha, Qiaozhi
(author)
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Carslaw, Kenneth S.
(author)
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Curtius, Joachim
(author)
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Donahue, Neil M.
(author)
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Flagan, Richard C.
(author)
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Hansel, Armin
(author)
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Riipinen, IlonaStockholms universitet,Institutionen för miljövetenskap och analytisk kemi,Tampere University of Technology, Finland(Swepub:su)iriip
(author)
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Virtanen, Annele
(author)
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Winkler, Paul M.
(author)
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Baltensperger, Urs
(author)
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Kulmala, Markku
(author)
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Worsnop, Douglas R.
(author)
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Stockholms universitetInstitutionen för miljövetenskap och analytisk kemi
(creator_code:org_t)
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In:Science Advances: American Association for the Advancement of Science (AAAS)4:122375-2548
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- By the author/editor
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Lehtipalo, Katri ...
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Yan, Chao
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Dada, Lubna
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Bianchi, Federic ...
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Xiao, Mao
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Wagner, Robert
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show more...
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Stolzenburg, Dom ...
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Ahonen, Lauri R.
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Amorim, Antonio
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Baccarini, Andre ...
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Bauer, Paulus S.
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Baumgartner, Ber ...
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Bergen, Anton
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Bernhammer, Anne ...
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Breitenlechner, ...
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Brilke, Sophia
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Buchholz, Angela
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Mazon, Stephany ...
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Chen, Dexian
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Chen, Xuemeng
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Dias, Antonio
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Dommen, Josef
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Draper, Danielle ...
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Duplissy, Jonath ...
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Ehn, Mikael
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Finkenzeller, He ...
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Fischer, Lukas
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Frege, Carla
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Fuchs, Claudia
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Garmash, Olga
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Gordon, Hamish
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Hakala, Jani
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He, Xucheng
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Heikkinen, Liine
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Heinritzi, Marti ...
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Helm, Johanna C.
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Hofbauer, Victor ...
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Hoyle, Christoph ...
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Jokinen, Tuija
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Kangasluoma, Juh ...
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Kerminen, Veli-M ...
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Kim, Changhyuk
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Kirkby, Jasper
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Kontkanen, Jenni
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Kuerten, Andreas
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Lawler, Michael ...
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Mai, Huajun
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Mathot, Serge
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Mauldin, Roy L.
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Molteni, Ugo
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Nichman, Leonid
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Nie, Wei
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Nieminen, Tuomo
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Ojdanic, Andrea
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Onnela, Antti
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Passananti, Moni ...
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Petaja, Tuukka
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Piel, Felix
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Pospisilova, Ver ...
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Quelever, Lauria ...
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Rissanen, Matti ...
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Rose, Clemence
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Sarnela, Nina
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Schallhart, Simo ...
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Schuchmann, Simo ...
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Sengupta, Kamali ...
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Simon, Mario
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Sipila, Mikko
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Tauber, Christia ...
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Tome, Antonio
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Trostl, Jasmin
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Vaisanen, Olli
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Vogel, Alexander ...
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Volkamer, Rainer
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Wagner, Andrea C ...
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Wang, Mingyi
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Weitz, Lena
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Wimmer, Daniela
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Ye, Penglin
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Ylisirnio, Arttu
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Zha, Qiaozhi
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Carslaw, Kenneth ...
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Curtius, Joachim
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Donahue, Neil M.
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Flagan, Richard ...
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Hansel, Armin
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Riipinen, Ilona
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Virtanen, Annele
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Winkler, Paul M.
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Baltensperger, U ...
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Kulmala, Markku
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Stockholm University