Sökning: WFRF:(Tchaplyguine M.) > (2010-2014) > Size-dependent evol...
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000 | 03270naa a2200493 4500 | |
001 | oai:lup.lub.lu.se:72e47cca-57c3-4ca0-8f61-50a4d11ea92f | |
003 | SwePub | |
008 | 160401s2014 | |||||||||||000 ||eng| | |
009 | oai:DiVA.org:uu-236100 | |
024 | 7 | a https://lup.lub.lu.se/record/48003902 URI |
024 | 7 | a https://doi.org/10.1016/j.elspec.2014.05.0112 DOI |
024 | 7 | a https://urn.kb.se/resolve?urn=urn:nbn:se:uu:diva-2361002 URI |
040 | a (SwePub)lud (SwePub)uu | |
041 | a engb eng | |
042 | 9 SwePub | |
072 | 7 | a art2 swepub-publicationtype |
072 | 7 | a ref2 swepub-contenttype |
100 | 1 | a Tchaplyguine, Maximu Lund University,Lunds universitet,MAX IV-laboratoriet,MAX IV Laboratory4 aut0 (Swepub:lu)maxl-mtc |
245 | 1 0 | a Size-dependent evolution of electronic structure in neutral Pb clusters-As seen by synchrotron-based X-ray photoelectron spectroscopy |
264 | 1 | b Elsevier BV,c 2014 |
520 | a Neutral Pb clusters in the size range from a few tens of atoms up to similar to 100 atoms are studied using synchrotron-based photoelectron spectroscopy. The electronic structure is seen to differ increasingly from that of the solid when the cluster size decreases. The valence band narrows gradually - down to about one fifth of the solid-state band width at the smallest size of few tens of atoms. Simultaneously the Fermi-edge energy shifts further away from the solid value by more than 2 eV. The Pb 5d core level binding energy also increases and the spectral features broaden and change in shape. The changes observed for the valence and for the 5d response energies and shapes are discussed in the context of the metal-to-insulator transition observed earlier in Pb clusters below the critical size of 20-30 atoms/cluster. (C) 2014 Elsevier B.V. All rights reserved. | |
650 | 7 | a NATURVETENSKAPx Fysik0 (SwePub)1032 hsv//swe |
650 | 7 | a NATURAL SCIENCESx Physical Sciences0 (SwePub)1032 hsv//eng |
653 | a Metal clusters | |
653 | a Photoelectron spectroscopy | |
653 | a Synchrotron radiation | |
653 | a Metal clusters | |
700 | 1 | a Öhrwall, Gunnaru Lund University,Lunds universitet,MAX IV-laboratoriet,MAX IV Laboratory4 aut0 (Swepub:lu)maxl-goh |
700 | 1 | a Andersson, T.u Uppsala universitet,Institutionen för fysik och astronomi4 aut |
700 | 1 | a Svensson, Svanteu Uppsala universitet,Molekyl- och kondenserade materiens fysik,Institutionen för fysik och astronomi4 aut0 (Swepub:uu)svansven |
700 | 1 | a Björneholm, Olle4 aut |
700 | 1 | a Huttula, M.4 aut |
700 | 1 | a Mikkela, M.4 aut |
700 | 1 | a Urpelainen, Samuliu Lund University,Lunds universitet,MAX IV-laboratoriet,MAX IV Laboratory4 aut0 (Swepub:lu)maxl-sua |
700 | 1 | a Osmekhin, S.4 aut |
700 | 1 | a Calo, A.4 aut |
700 | 1 | a Aksela, S.4 aut |
700 | 1 | a Aksela, H.4 aut |
710 | 2 | a Lunds universitetb MAX IV-laboratoriet4 org |
773 | 0 | t Journal of Electron Spectroscopy and Related Phenomenad : Elsevier BVg 195, s. 55-61q 195<55-61x 0368-2048x 1873-2526 |
856 | 4 | u http://dx.doi.org/10.1016/j.elspec.2014.05.011y FULLTEXT |
856 | 4 8 | u https://lup.lub.lu.se/record/4800390 |
856 | 4 8 | u https://doi.org/10.1016/j.elspec.2014.05.011 |
856 | 4 8 | u https://urn.kb.se/resolve?urn=urn:nbn:se:uu:diva-236100 |
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