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X-ray laser-induced ablation of lead compounds

Hajkova, V. (author)
Juha, L. (author)
Bohacek, P. (author)
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Burian, T. (author)
Chalupsky, J. (author)
Vysin, L. (author)
Gaudin, J. (author)
Heimann, P. A. (author)
Hau-Riege, S. P. (author)
Jurek, M. (author)
Klinger, D. (author)
Pelka, J. (author)
Sobierajski, R. (author)
Krzywinski, J. (author)
Messerschmidt, M. (author)
Moeller, S. P. (author)
Nagler, B. (author)
Rowen, M. (author)
Schlotter, W. F. (author)
Swiggers, M. L. (author)
Turner, J. J. (author)
Vinko, S. M. (author)
Whitcher, T. (author)
Wark, J. (author)
Matuchova, M. (author)
Bajt, S. (author)
Chapman, H. (author)
Dzelzainis, T. (author)
Riley, D. (author)
Andreasson, J. (author)
Uppsala universitet,Molekylär biofysik
Hajdu, J. (author)
Uppsala universitet,Molekylär biofysik
Iwan, B. (author)
Uppsala universitet,Molekylär biofysik
Timneanu, N. (author)
Uppsala universitet,Molekylär biofysik
Saksl, K. (author)
Faeustlin, R. (author)
Singer, A. (author)
Tiedtke, K. (author)
Toleikis, S. (author)
Vartaniants, I. (author)
Wabnitz, H. (author)
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 (creator_code:org_t)
SPIE, 2011
2011
English.
In: DAMAGE TO VUV, EUV, AND X-RAY OPTICS III. - : SPIE.
  • Conference paper (peer-reviewed)
Abstract Subject headings
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  • The recent commissioning of a X-ray free-electron laser triggered an extensive research in the area of X-ray ablation of high-Z, high-density materials. Such compounds should be used to shorten an effective attenuation length for obtaining clean ablation imprints required for the focused beam analysis. Compounds of lead (Z=82) represent the materials of first choice. In this contribution, single-shot ablation thresholds are reported for PbWO(4) and PbI(2) exposed to ultra-short pulses of extreme ultraviolet radiation and X-rays at FLASH and LCLS facilities, respectively. Interestingly, the threshold reaches only 0.11 J/cm(2) at 1.55 nm in lead tungstate although a value of 0.4 J/cm(2) is expected according to the wavelength dependence of an attenuation length and the threshold value determined in the XUV spectral region, i.e., 79 mJ/cm(2) at a FEL wavelength of 13.5 nm. Mechanisms of ablation processes are discussed to explain this discrepancy. Lead iodide shows at 1.55 nm significantly lower ablation threshold than tungstate although an attenuation length of the radiation is in both materials quite the same. Lower thermal and radiation stability of PbI(2) is responsible for this finding.

Subject headings

NATURVETENSKAP  -- Fysik -- Annan fysik (hsv//swe)
NATURAL SCIENCES  -- Physical Sciences -- Other Physics Topics (hsv//eng)

Keyword

extreme ultraviolet laser; x-ray laser; free-electron laser; radiation damage; laser ablation; damage thresholds; single-shot damage; focused beam characterization

Publication and Content Type

ref (subject category)
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