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LIBRIS Formathandbok  (Information om MARC21)
FältnamnIndikatorerMetadata
00008083naa a2200649 4500
001oai:DiVA.org:umu-189888
003SwePub
008211125s2022 | |||||||||||000 ||eng|
009oai:DiVA.org:uu-473565
009oai:DiVA.org:liu-184527
0247 a https://urn.kb.se/resolve?urn=urn:nbn:se:umu:diva-1898882 URI
0247 a https://doi.org/10.1016/j.cej.2021.1331902 DOI
0247 a https://urn.kb.se/resolve?urn=urn:nbn:se:uu:diva-4735652 URI
0247 a https://urn.kb.se/resolve?urn=urn:nbn:se:liu:diva-1845272 URI
040 a (SwePub)umud (SwePub)uud (SwePub)liu
041 a engb eng
042 9 SwePub
072 7a ref2 swepub-contenttype
072 7a art2 swepub-publicationtype
1001 a Zhao, Xueu Institute for Ecological Research and Pollution Control of Plateau Lakes, School of Ecology and Environmental Science, Yunnan University, Kunming, China; College of Chemistry and Molecular Sciences, Wuhan University, Wuhan, China,Yunnan Univ, Sch Ecol & Environm Sci, Inst Ecol Res & Pollut Control Plateau Lakes, Kunming 650504, Yunnan, Peoples R China.;Wuhan Univ, Coll Chem & Mol Sci, Wuhan 430072, Peoples R China.4 aut
2451 0a Simultaneous anchoring of Ni nanoparticles and single-atom Ni on BCN matrix promotes efficient conversion of nitrate in water into high-value-added ammonia
264 1b Elsevier,c 2022
338 a print2 rdacarrier
500 a Funding Agencies|National Key Research and Development Program of China [2019YFC1804400]; Special Project for Social Development of Yunnan Province [202103AC100001]; National Natural Science Foundation of ChinaNational Natural Science Foundation of China (NSFC) [U2002213, 22179100]; Yunnan Science and Technology Bureau [2019FY003025]; Yunnan University [2019FY003025]; Double-First Class University Construction Project [C176220100042]; science and technology innovation Program of Hunan Province [2020RC5026, 2020GK4040]; Swedish Research CouncilSwedish Research CouncilEuropean Commission [2020-04600, SNIC 2020/329]; Olle Engkvist Byggmastare foundation [212-0178]
520 a Electrochemical synthesis of ammonia driven by clean energy is expected to realize the supply of ammonia for distributed production of industry and agriculture. Here, nickel nanoparticles and nickel in the form of single atoms were simultaneously anchored on the electrochemically active carrier BCN matrix through a structured domain strategy, which realized a high-efficiency, high-value-added, conversion of nitrate in sewage. Specifically, the electrochemical nitrate reduction reaction (NIRR) driven by BCN@Ni in alkaline media achieves an ammonia yield rate as high as 2320.2 μg h−1 cm−2 (at −0.5 V vs RHE), and Faraday efficiency as high as 91.15% (at −0.3 V vs RHE). Even in neutral and acidic media, the ammonia yield rates of NIRR driven by BCN@Ni are as high as 1904.2 μg h−1 cm−2 and 2057.4 μg h−1 cm−2, respectively (at −0.4 V vs RHE). The 15NO3- isotope labeling experiment verified that the recorded ammonia all came from the electrochemical reduction of NO3– on BCN@Ni. Density functional theory (DFT) calculations show that both nano-Ni and single-atom Ni in BCN@Ni have the ability to electrochemically convert NO3– into NH3, and that the addition of BCN can further promote the NIRR on Ni.
650 7a NATURVETENSKAPx Kemix Fysikalisk kemi0 (SwePub)104022 hsv//swe
650 7a NATURAL SCIENCESx Chemical Sciencesx Physical Chemistry0 (SwePub)104022 hsv//eng
650 7a NATURVETENSKAPx Kemix Materialkemi0 (SwePub)104032 hsv//swe
650 7a NATURAL SCIENCESx Chemical Sciencesx Materials Chemistry0 (SwePub)104032 hsv//eng
650 7a NATURVETENSKAPx Kemix Organisk kemi0 (SwePub)104052 hsv//swe
650 7a NATURAL SCIENCESx Chemical Sciencesx Organic Chemistry0 (SwePub)104052 hsv//eng
653 a Ammonia energy
653 a Electrocatalysis
653 a Nitrate reduction
653 a Sewage purification
653 a Single-atom Ni
653 a Synthetic ammonia
7001 a Zhu, Zhuu Institute for Ecological Research and Pollution Control of Plateau Lakes, School of Ecology and Environmental Science, Yunnan University, Kunming, China,Yunnan Univ, Sch Ecol & Environm Sci, Inst Ecol Res & Pollut Control Plateau Lakes, Kunming 650504, Yunnan, Peoples R China.,Wuhan Univ, Coll Chem & Mol Sci, Wuhan 430072, Peoples R China.4 aut
7001 a He, Yingnanu Institute for Ecological Research and Pollution Control of Plateau Lakes, School of Ecology and Environmental Science, Yunnan University, Kunming, China,Yunnan Univ, Sch Ecol & Environm Sci, Inst Ecol Res & Pollut Control Plateau Lakes, Kunming 650504, Yunnan, Peoples R China.4 aut
7001 a Zhang, Haibou College of Chemistry and Molecular Sciences, Wuhan University, Wuhan, China,Wuhan Univ, Coll Chem & Mol Sci, Wuhan 430072, Peoples R China.4 aut
7001 a Zhou, Xiaohaiu College of Chemistry and Molecular Sciences, Wuhan University, Wuhan, China4 aut
7001 a Hu, Wanbiaou Institute for Ecological Research and Pollution Control of Plateau Lakes, School of Ecology and Environmental Science, Yunnan University, Kunming, China,Yunnan Univ, Sch Ecol & Environm Sci, Inst Ecol Res & Pollut Control Plateau Lakes, Kunming 650504, Yunnan, Peoples R China.4 aut
7001 a Li, Mengu College of Chemistry and Molecular Engineering, Zhengzhou University, Zhengzhou, China,Zhengzhou Univ, Coll Chem & Mol Engn, Zhengzhou 450000, Peoples R China.4 aut
7001 a Zhang, Shushengu College of Chemistry and Molecular Engineering, Zhengzhou University, Zhengzhou, China,Zhengzhou Univ, Coll Chem & Mol Engn, Zhengzhou 450000, Peoples R China.4 aut
7001 a Dong, Yeminu State Key Laboratory of Functional Materials for Informatics, Shanghai Institute of Microsystem and Information Technology, Chinese Academy of Sciences, Shanghai, China,Chinese Acad Sci, Shanghai Inst Microsyst & Informat Technol, State Key Lab Funct Mat Informat, Shanghai 200050, Peoples R China.4 aut
7001 a Hu, Xunu School of Materials Science and Engineering, University of Jinan, Jinan, China,Univ Jinan, Sch Mat Sci & Engn, Jinan 250022, Peoples R China.4 aut
7001 a Kuklin, Artem V.u Uppsala universitet,Institutionen för fysik och astronomi,Siberian Fed Univ, Int Res Ctr Spect & Quantum Chem IRC SQC, 79 Svobodny Pr, Krasnoyarsk 660041, Russia.,Röntgenfysik,Siberian Fed Univ, Russia; Uppsala Univ, Sweden4 aut0 (Swepub:uu)artku415
7001 a Baryshnikov, Glibu Linköpings universitet,Laboratoriet för organisk elektronik,Tekniska fakulteten4 aut0 (Swepub:liu)gliba58
7001 a Ågren, Hansu Uppsala universitet,Institutionen för fysik och astronomi,Röntgenfysik,Uppsala Univ, Sweden4 aut0 (Swepub:uu)hanag788
7001 a Wågberg, Thomas,d 1971-u Umeå universitet,Institutionen för fysik,Umeå Univ, Dept Phys, SE-90187 Umeå, Sweden.4 aut0 (Swepub:umu)thwa0002
7001 a Hu, Guangzhiu Institute for Ecological Research and Pollution Control of Plateau Lakes, School of Ecology and Environmental Science, Yunnan University, Kunming, China,Yunnan Univ, Sch Ecol & Environm Sci, Inst Ecol Res & Pollut Control Plateau Lakes, Kunming 650504, Yunnan, Peoples R China.4 aut
7102 a Institute for Ecological Research and Pollution Control of Plateau Lakes, School of Ecology and Environmental Science, Yunnan University, Kunming, China; College of Chemistry and Molecular Sciences, Wuhan University, Wuhan, Chinab Yunnan Univ, Sch Ecol & Environm Sci, Inst Ecol Res & Pollut Control Plateau Lakes, Kunming 650504, Yunnan, Peoples R China.;Wuhan Univ, Coll Chem & Mol Sci, Wuhan 430072, Peoples R China.4 org
7730 t Chemical Engineering Journald : Elsevierg 433:Part 2q 433:Part 2x 1385-8947x 1873-3212
8564 8u https://urn.kb.se/resolve?urn=urn:nbn:se:umu:diva-189888
8564 8u https://doi.org/10.1016/j.cej.2021.133190
8564 8u https://urn.kb.se/resolve?urn=urn:nbn:se:uu:diva-473565
8564 8u https://urn.kb.se/resolve?urn=urn:nbn:se:liu:diva-184527

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