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Generation of intense phase-stable femtosecond hard X-ray pulse pairs

Zhang, Yu (author)
Stanford Linear Accelerator Center (SLAC)
Kroll, Thomas (author)
Stanford Linear Accelerator Center (SLAC)
Weninger, Clemens (author)
Lund University,Lunds universitet,MAX IV-laboratoriet,MAX IV Laboratory,Stanford Linear Accelerator Center (SLAC)
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Michine, Yurina (author)
University of Electro-Communications
Fuller, Franklin D. (author)
Stanford Linear Accelerator Center (SLAC)
Zhu, Diling (author)
Stanford Linear Accelerator Center (SLAC)
Alonso-Mori, Roberto (author)
Stanford Linear Accelerator Center (SLAC)
Sokaras, Dimosthenis (author)
Stanford Linear Accelerator Center (SLAC)
Lutman, Alberto A. (author)
Stanford Linear Accelerator Center (SLAC)
Halavanau, Aliaksei (author)
Stanford Linear Accelerator Center (SLAC)
Pellegrini, Claudio (author)
Stanford Linear Accelerator Center (SLAC)
Benediktovitch, Andrei (author)
German Electron Synchrotron (DESY)
Yabashi, Makina (author)
Japan Synchrotron Radiation Research Institute,RIKEN SPring-8 center
Inoue, Ichiro (author)
RIKEN SPring-8 center
Inubushi, Yuichi (author)
RIKEN SPring-8 center,Japan Synchrotron Radiation Research Institute
Osaka, Taito (author)
RIKEN SPring-8 center
Yamada, Jumpei (author)
RIKEN SPring-8 center
Babu, Ganguli (author)
Rice University
Salpekar, Devashish (author)
Rice University
Sayed, Farheen N. (author)
Rice University
Ajayan, Pulickel M. (author)
Rice University
Kern, Jan (author)
Lawrence Berkeley National Laboratory
Yano, Junko (author)
Lawrence Berkeley National Laboratory
Yachandra, Vittal K. (author)
Lawrence Berkeley National Laboratory
Yoneda, Hitoki (author)
University of Electro-Communications
Rohringer, Nina (author)
University of Hamburg,German Electron Synchrotron (DESY)
Bergmann, Uwe (author)
Stanford Linear Accelerator Center (SLAC),University of Wisconsin-Madison
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 (creator_code:org_t)
2022-03-15
2022
English.
In: Proceedings of the National Academy of Sciences of the United States of America. - : Proceedings of the National Academy of Sciences. - 0027-8424. ; 119:12
  • Journal article (peer-reviewed)
Abstract Subject headings
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  • Coherent nonlinear spectroscopies and imaging in the X-ray domain provide direct insight into the coupled motions of electrons and nuclei with resolution on the electronic length scale and timescale. The experimental realization of such techniques will strongly benefit from access to intense, coherent pairs of femtosecond X-ray pulses. We have observed phase-stable X-ray pulse pairs containing more than 3 × 107 photons at 5.9 keV (2.1 Å) with ∼1 fs duration and 2 to 5 fs separation. The highly directional pulse pairs are manifested by interference fringes in the superfluorescent and seeded stimulated manganese Kα emission induced by an X-ray free-electron laser. The fringes constitute the time-frequency X-ray analog of Young’s double-slit interference, allowing for frequency domain X-ray measurements with attosecond time resolution.

Subject headings

NATURVETENSKAP  -- Fysik -- Atom- och molekylfysik och optik (hsv//swe)
NATURAL SCIENCES  -- Physical Sciences -- Atom and Molecular Physics and Optics (hsv//eng)

Keyword

Frequency combs
Interferometry
X-rays sciences

Publication and Content Type

art (subject category)
ref (subject category)

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