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Sökning: WFRF:(Yang Jinman) > (2021) > Accelerated Photore...

LIBRIS Formathandbok  (Information om MARC21)
FältnamnIndikatorerMetadata
00004396naa a2200457 4500
001oai:DiVA.org:liu-179621
003SwePub
008210929s2021 | |||||||||||000 ||eng|
024a https://urn.kb.se/resolve?urn=urn:nbn:se:liu:diva-1796212 URI
024a https://doi.org/10.1021/acsami.1c126922 DOI
040 a (SwePub)liu
041 a engb eng
042 9 SwePub
072 7a ref2 swepub-contenttype
072 7a art2 swepub-publicationtype
100a Zhu, Xingwangu Jiangsu Univ, Peoples R China; Natl Univ Singapore, Singapore4 aut
2451 0a Accelerated Photoreduction of CO2 to CO over a Stable Heterostructure with a Seamless Interface
264 c 2021-08-13
264 1b AMER CHEMICAL SOC,c 2021
338 a print2 rdacarrier
500 a Funding Agencies|National Natural Science Foundation of ChinaNational Natural Science Foundation of China (NSFC) [22075113, 22005123]; Jiangsu Fund for Distinguished Young Scientists [BK20190045]; Natural Science Foundation of Jiangsu ProvinceNatural Science Foundation of Jiangsu Province [BK20190981]; Hightech Research Key Laboratory of Zhenjiang [SS2018002]; China Postdoctoral Science FoundationChina Postdoctoral Science Foundation [2019M661765]; Jiangsu Provincial Agricultural Science and Technology Independent Innovation Fund [CX(20)3081]; Key Laboratory of Electrochemical Energy Storage and Energy Conversion of Hainan Province [KFKT2019002]; Jiangsu Government Scholarship for Overseas Studies [JS-2020-203]; Priority Academic Program Development of Jiangsu Higher Education Institutions; HighPerformance Computing Platform of Jiangsu University; Jiangsu University Study-abroad Scholarship for Overseas Study [UJS-2020-001]
520 a Photocatalytic CO2 reduction is a means of alleviating energy crisis and environmental deterioration. In this work, a rising two-dimensional (2D) material rarely reported in the field of photocatalytic CO2 reduction, black phosphorus (BP) nanosheets, is synthesized, on which Co2P is in situ grown by solvothermal treatment using BP itself as a P source. Co2P on the BP nanosheets (BPs) surface can prevent the destruction of BPs in ambient air and, in the meantime, favor charge separation and CO2 adsorption and activation during the catalytic process. Upon light irradiation, Co2P can extract the photogenerated electrons effectively across the intimate interface and lower the CO2 activation energy barrier, supported by both experimental characterizations and theoretical calculations. Benefitting from integrated advantages of BPs and Co2P, the optimal Co2P/BPs exhibit photocatalytic reduction of CO2 to CO at a rate of 25.5 mu mol g(-1) h(-1) with a selectivity of 91.4%, both of which are higher than those of pristine BPs. This work presents ideas for stabilizing BPs and improving their CO2 reduction performance simultaneously.
650 7a NATURVETENSKAPx Kemix Materialkemi0 (SwePub)104032 hsv//swe
650 7a NATURAL SCIENCESx Chemical Sciencesx Materials Chemistry0 (SwePub)104032 hsv//eng
653 a CO2 conversion; black phosphorus; Co2P; photocatalyst; charge transfer; interface; 2D material
700a Zhou, Guliu Jiangsu Univ, Peoples R China4 aut
700a Yi, Jianjianu Yangzhou Univ, Peoples R China4 aut
700a Ding, Penghuiu Linköpings universitet,Laboratoriet för organisk elektronik,Tekniska fakulteten4 aut0 (Swepub:liu)pendi14
700a Yang, Jinmanu Jiangsu Univ, Peoples R China4 aut
700a Zhong, Kangu Jiangsu Univ, Peoples R China4 aut
700a Song, Yanhuau Jiangsu Univ Sci & Technol, Peoples R China4 aut
700a Hua, Yingjieu Hainan Normal Univ, Peoples R China4 aut
700a Zhu, Xianglinu Jiangsu Univ, Peoples R China4 aut
700a Yuan, Junjieu Jiangsu Univ, Peoples R China4 aut
700a She, Yuanbinu Zhejiang Univ Technol, Peoples R China4 aut
700a Li, Huamingu Jiangsu Univ, Peoples R China4 aut
700a Xu, Huiu Jiangsu Univ, Peoples R China4 aut
710a Jiangsu Univ, Peoples R China; Natl Univ Singapore, Singaporeb Jiangsu Univ, Peoples R China4 org
773t ACS Applied Materials and Interfacesd : AMER CHEMICAL SOCg 13:33, s. 39523-39532q 13:33<39523-39532x 1944-8244x 1944-8252
8564 8u https://urn.kb.se/resolve?urn=urn:nbn:se:liu:diva-179621
8564 8u https://doi.org/10.1021/acsami.1c12692

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