L773:1369 9261 OR L773:1144 0546
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Catalysed low temperature H-2 release from nitrogen heterocycles
- Moores, Audrey (author)
- Poyatos, Macarena (author)
-
- Luo, Yi (author)
- KTH,Teoretisk kemi
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- Crabtree, Robert H. (author)
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- (creator_code:org_t)
- Royal Society of Chemistry (RSC), 2006
- 2006
- English.
- In: New Journal of Chemistry. - : Royal Society of Chemistry (RSC). - 1144-0546 .- 1369-9261. ; 30:11, s. 1675-1678
- Journal article (peer-reviewed)
Abstract
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- In an experimental and computational study, nitrogen- and oxygen-containing heterocycles were compared with carbocycles as liquid substrates for hydrogen release with heterogeneous catalysts. Heteroatom substitution, particularly by nitrogen, favours low temperature H-2 release; indoline was fully dehydrogenated in less than 30 min with Pd/C at 110 degrees C.
Keyword
- molecular-orbital methods
- noble-metal catalysts
- carbon nanotubes
- dehydrogenation
- hydrogen
- storage
- complexes
- evolution
- energies
- alcohols
Publication and Content Type
- ref (subject category)
- art (subject category)
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