Non-fullerene acceptor photostability and its impact on organic solar cell lifetime

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Fältnamn	Indikatorer	Metadata
000		05119naa a2200553 4500
001		oai:DiVA.org:liu-178475
003		SwePub
008		210825s2021 \| \|\|\|\|\|\|\|\|\|\|\|000 \|\|eng\|
024	7	a https://urn.kb.se/resolve?urn=urn:nbn:se:liu:diva-1784752 URI
024	7	a https://doi.org/10.1016/j.xcrp.2021.1004982 DOI
040		a (SwePub)liu
041		a engb eng
042		9 SwePub
072	7	a ref2 swepub-contenttype
072	7	a art2 swepub-publicationtype
100	1	a Clarke, Andrew J.u Swansea Univ, Wales4 aut
245	1 0	a Non-fullerene acceptor photostability and its impact on organic solar cell lifetime
264	1	b Elsevier,c 2021
338		a electronic2 rdacarrier
500		a Funding Agencies\|European Social Fund via the Welsh Government; EPSRCUK Research & Innovation (UKRI)Engineering & Physical Sciences Research Council (EPSRC) [EP/L015099/1, EP/T026219/1, EP/S020748/1]; UK EPSRCUK Research & Innovation (UKRI)Engineering & Physical Sciences Research Council (EPSRC) [EP/L016702/1]; ATIP Programme grant [EP/T028513/1]; CSEM Brasil; Global Research Laboratory Program of the National Research Foundation (NRF) - Ministry of Science, ICT & Future Planning [NRF-2017K1A1A2013153]; UKRI Global Challenge Research Fund project, SUNRISE [EP/P032591/1]; Office of Sponsored Research (OSR) [OSR-2018-CRG/CCF-3079, OSR-2019-CRG8-4086, OSR-2018-CRG7-3749]; European Social Fund, European Union CSEM Brasil, Brazil European Research Council, European Union ERC Synergy Grant [SC2 (610115)]; European Unions Horizon 2020 research and innovation programme [952911]; project BOOSTER [862474]; project RoLA-FLEX; KAUSTKing Abdullah University of Science & Technology
520		a The development of non-fullerene acceptors (NFAs) has facilitated the realization of efficient organic solar cells (OSCs) with minimal burn-in losses and excellent long-term stability. However, the role of NFA molecular structures on device stability remains unclear, limiting commercialization of NFA-based OSCs. Herein, the photostability of 10 OSC devices, fabricated with various NFAs (O-IDTBR, EH-IDTBR, ITIC, and ITIC-M) blended with donor polymers (PTB7-Th, PffBT4T-2OD, and PBDB-T), is investigated. O-IDTBR and EH-IDTBR form highly stable devices with all three polymers, whereas ITIC and ITIC-M devices suffer from burn-in losses and long-term degradation. Conformational instability is found to be responsible for the poor photostability of ITIC and ITIC-M, resulting in poor device stability. Twisting and potential breakage of the chemical bond that links the end group to the main backbone of ITIC and ITIC-M molecules causes undesirable conformational changes. Potential strategies to overcome such detrimental photo-induced conformational changes in NFAs are proposed.
650	7	a NATURVETENSKAPx Kemix Polymerkemi0 (SwePub)104062 hsv//swe
650	7	a NATURAL SCIENCESx Chemical Sciencesx Polymer Chemistry0 (SwePub)104062 hsv//eng
700	1	a Luke, Joelu Imperial Coll London, England; Imperial Coll London, England4 aut
700	1	a Meitzner, Ricou Friedrich Schiller Univ Jena, Germany4 aut
700	1	a Wu, Jiayingu Imperial Coll London, England; Imperial Coll London, England4 aut
700	1	a Wang, Yumingu Linköpings universitet,Elektroniska och fotoniska material,Tekniska fakulteten4 aut0 (Swepub:liu)yumwa29
700	1	a Lee, Harrison K. H.u Swansea Univ, Wales4 aut
700	1	a Speller, Emily M.u Swansea Univ, Wales4 aut
700	1	a Bristow, Helenu Univ Oxford, England4 aut
700	1	a Cha, Hyojungu Imperial Coll London, England; Imperial Coll London, England4 aut
700	1	a Newman, Michael J.u Swansea Univ, Wales4 aut
700	1	a Hooper, Katherineu Swansea Univ, Wales4 aut
700	1	a Evans, Alexu Cardiff Univ, Wales4 aut
700	1	a Gao, Fengu Linköpings universitet,Elektroniska och fotoniska material,Tekniska fakulteten4 aut0 (Swepub:liu)fenga88
700	1	a Hoppe, Haraldu Friedrich Schiller Univ Jena, Germany4 aut
700	1	a McCulloch, Iainu Univ Oxford, England; King Abdullah Univ Sci & Technol KAUST, Saudi Arabia4 aut
700	1	a Schubert, Ulrich S.u Friedrich Schiller Univ Jena, Germany; Friedrich Schiller Univ Jena, Germany4 aut
700	1	a Watson, Trystan M.u Swansea Univ, Wales4 aut
700	1	a Durrant, James R.u Swansea Univ, Wales; Imperial Coll London, England; Imperial Coll London, England4 aut
700	1	a Tsoi, Wing C.u Swansea Univ, Wales4 aut
700	1	a Kim, Ji-Seonu Imperial Coll London, England; Imperial Coll London, England4 aut
700	1	a Li, Zheu Queen Mary Univ London, England4 aut
710	2	a Swansea Univ, Walesb Imperial Coll London, England; Imperial Coll London, England4 org
773	0	t Cell Reports Physical Scienced : Elsevierg 2:7q 2:7x 2666-3864
856	4	u https://liu.diva-portal.org/smash/get/diva2:1587625/FULLTEXT01.pdfx primaryx Raw objecty fulltext:print
856	4	u https://doi.org/10.1016/j.xcrp.2021.100498
856	4 8	u https://urn.kb.se/resolve?urn=urn:nbn:se:liu:diva-178475
856	4 8	u https://doi.org/10.1016/j.xcrp.2021.100498

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