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Observation of Pore Growth and Self-Organization in Anodic Alumina by Time-Resolved X-ray Scattering

Vinogradov, Nikolay A. (författare)
Lund University,Lunds universitet,MAX IV-laboratoriet,MAX IV Laboratory
Harlow, Gary S. (författare)
Lund University,Lunds universitet,NanoLund: Centre for Nanoscience,Annan verksamhet, LTH,Lunds Tekniska Högskola,Synkrotronljusfysik,Fysiska institutionen,Institutioner vid LTH,Other operations, LTH,Faculty of Engineering, LTH,Synchrotron Radiation Research,Department of Physics,Departments at LTH,Faculty of Engineering, LTH
Carlà, Francesco (författare)
European Synchrotron Radiation Facility
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Evertsson, Jonas (författare)
Lund University,Lunds universitet,NanoLund: Centre for Nanoscience,Annan verksamhet, LTH,Lunds Tekniska Högskola,Synkrotronljusfysik,Fysiska institutionen,Institutioner vid LTH,Other operations, LTH,Faculty of Engineering, LTH,Synchrotron Radiation Research,Department of Physics,Departments at LTH,Faculty of Engineering, LTH
Rullik, Lisa (författare)
Lund University,Lunds universitet,NanoLund: Centre for Nanoscience,Annan verksamhet, LTH,Lunds Tekniska Högskola,Synkrotronljusfysik,Fysiska institutionen,Institutioner vid LTH,Other operations, LTH,Faculty of Engineering, LTH,Synchrotron Radiation Research,Department of Physics,Departments at LTH,Faculty of Engineering, LTH
Linpé, Weronica (författare)
Lund University,Lunds universitet,NanoLund: Centre for Nanoscience,Annan verksamhet, LTH,Lunds Tekniska Högskola,Synkrotronljusfysik,Fysiska institutionen,Institutioner vid LTH,Other operations, LTH,Faculty of Engineering, LTH,Synchrotron Radiation Research,Department of Physics,Departments at LTH,Faculty of Engineering, LTH
Felici, Roberto (författare)
European Synchrotron Radiation Facility
Lundgren, Edvin (författare)
Lund University,Lunds universitet,NanoLund: Centre for Nanoscience,Annan verksamhet, LTH,Lunds Tekniska Högskola,Synkrotronljusfysik,Fysiska institutionen,Institutioner vid LTH,Other operations, LTH,Faculty of Engineering, LTH,Synchrotron Radiation Research,Department of Physics,Departments at LTH,Faculty of Engineering, LTH
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 (creator_code:org_t)
2018-03-01
2018
Engelska 7 s.
Ingår i: ACS Applied Nano Materials. - : American Chemical Society (ACS). - 2574-0970. ; 1:3, s. 1265-1271
  • Tidskriftsartikel (refereegranskat)
Abstract Ämnesord
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  • The anodic oxidation of metals such as aluminum and titanium can lead to the development of self-ordering pores. These pores make excellent templates for a range of nanoscale objects with many applications in nanoscience. Theoretical studies on pore formation have proposed several models for the establishment, growth, and ordering of these pores; however, experimental verification has mostly been limited to ex situ measurements. Here we show that the lateral and vertical pore structure can be probed in situ with high precision, using grazing transmission X-ray scattering. By making use of the high flux available at modern synchrotrons and fitting only the difference between scattering patterns we show the nearly real-time evolution of the pore’s arrangement. We observe no dependence on the substrate crystallographic orientation for domain size or pore separation. We do however observe an anisotropy in the oxide growth rate for the different substrate surfaces. This experimental approach can be applied to the study of a large variety of electrochemically produced materials such as magnetic nanowires, novel solar cell designs, and catalysts.

Ämnesord

NATURVETENSKAP  -- Fysik -- Den kondenserade materiens fysik (hsv//swe)
NATURAL SCIENCES  -- Physical Sciences -- Condensed Matter Physics (hsv//eng)

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