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Femtosecond x-ray photoelectron diffraction on gas-phase dibromobenzene molecules

Rolles, D. (author)
Boll, R. (author)
Adolph, M. (author)
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Aquila, A. (author)
Bostedt, C. (author)
Bozek, J. D. (author)
Chapman, H. N. (author)
Coffee, R. (author)
Coppola, N. (author)
Decleva, P. (author)
Delmas, T. (author)
Epp, S. W. (author)
Erk, B. (author)
Filsinger, F. (author)
Foucar, L. (author)
Gumprecht, L. (author)
Hoemke, A. (author)
Gorkhover, T. (author)
Holmegaard, L. (author)
Johnsson, Per (author)
Lund University,Lunds universitet,Atomfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Atomic Physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH
Kaiser, Ch (author)
Krasniqi, F. (author)
Kuehnel, K-U (author)
Maurer, J. (author)
Messerschmidt, M. (author)
Moshammer, R. (author)
Quevedo, W. (author)
Rajkovic, I. (author)
Rouzee, A. (author)
Rudek, B. (author)
Schlichting, I. (author)
Schmidt, C. (author)
Schorb, S. (author)
Schroeter, C. D. (author)
Schulz, J. (author)
Stapelfeldt, H. (author)
Stener, M. (author)
Stern, S. (author)
Techert, S. (author)
Thogersen, J. (author)
Vrakking, M. J. J. (author)
Rudenko, A. (author)
Kuepper, J. (author)
Ullrich, J. (author)
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 (creator_code:org_t)
2014-06-10
2014
English.
In: Journal of Physics B: Atomic, Molecular and Optical Physics. - : IOP Publishing. - 0953-4075 .- 1361-6455. ; 47:12
  • Journal article (peer-reviewed)
Abstract Subject headings
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  • We present time-resolved femtosecond photoelectron momentum images and angular distributions of dissociating, laser-aligned 1,4-dibromobenzene (C6H4Br2) molecules measured in a near-infrared pump, soft-x-ray probe experiment performed at an x-ray free-electron laser. The observed alignment dependence of the bromine 2p photoelectron angular distributions is compared to density functional theory calculations and interpreted in terms of photoelectron diffraction. While no clear time-dependent effects are observed in the angular distribution of the Br(2p) photoelectrons, other, low-energy electrons show a pronounced dependence on the time delay between the near-infrared laser and the x-ray pulse.

Subject headings

NATURVETENSKAP  -- Fysik -- Atom- och molekylfysik och optik (hsv//swe)
NATURAL SCIENCES  -- Physical Sciences -- Atom and Molecular Physics and Optics (hsv//eng)

Keyword

free-electron laser
photoelectron diffraction
molecular-frame
photoelectron angular distributions
laser alignment
femtosecond
pump-probe

Publication and Content Type

art (subject category)
ref (subject category)

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