Sökning: WFRF:(Janssen Stefan) > Improving Performan...
Fältnamn | Indikatorer | Metadata |
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000 | 04748naa a2200565 4500 | |
001 | oai:research.chalmers.se:da9c5ca5-06d5-4d2c-8464-e50175028d36 | |
003 | SwePub | |
008 | 181220s2018 | |||||||||||000 ||eng| | |
024 | 7 | a https://doi.org/10.1002/solr.2018002472 DOI |
024 | 7 | a https://research.chalmers.se/publication/5166762 URI |
024 | 7 | a https://research.chalmers.se/publication/5075312 URI |
040 | a (SwePub)cth | |
041 | a engb eng | |
042 | 9 SwePub | |
072 | 7 | a art2 swepub-publicationtype |
072 | 7 | a ref2 swepub-contenttype |
100 | 1 | a Duan, Chunhuiu Technische Universiteit Eindhoven,Eindhoven University of Technology,South China University of Technology4 aut |
245 | 1 0 | a Improving Performance of All-Polymer Solar Cells Through Backbone Engineering of Both Donors and Acceptors |
264 | c 2018-09-27 | |
264 | 1 | b Wiley,c 2018 |
338 | a electronic2 rdacarrier | |
520 | a All-polymer solar cells (APSCs), composed of semiconducting donor and acceptor polymers, have attracted considerable attention due to their unique advantages compared to polymer-fullerene-based devices in terms of enhanced light absorption and morphological stability. To improve the performance of APSCs, the morphology of the active layer must be optimized. By employing a random copolymerization strategy to control the regularity of the backbone of the donor polymers (PTAZ-TPDx) and acceptor polymers (PNDI-Tx) the morphology can be systematically optimized by tuning the polymer packing and crystallinity. To minimize effects of molecular weight, both donor and acceptor polymers have number-average molecular weights in narrow ranges. Experimental and coarse-grained modeling results disclose that systematic backbone engineering greatly affects the polymer crystallinity and ultimately the phase separation and morphology of the all-polymer blends. Decreasing the backbone regularity of either the donor or the acceptor polymer reduces the local crystallinity of the individual phase in blend films, affording reduced short-circuit current densities and fill factors. This two-dimensional crystallinity optimization strategy locates a PCE maximum at highest crystallinity for both donor and acceptor polymers. Overall, this study demonstrates that proper control of both donor and acceptor polymer crystallinity simultaneously is essential to optimize APSC performance. | |
650 | 7 | a NATURVETENSKAPx Kemix Polymerkemi0 (SwePub)104062 hsv//swe |
650 | 7 | a NATURAL SCIENCESx Chemical Sciencesx Polymer Chemistry0 (SwePub)104062 hsv//eng |
650 | 7 | a TEKNIK OCH TEKNOLOGIERx Kemiteknikx Polymerteknologi0 (SwePub)204032 hsv//swe |
650 | 7 | a ENGINEERING AND TECHNOLOGYx Chemical Engineeringx Polymer Technologies0 (SwePub)204032 hsv//eng |
650 | 7 | a TEKNIK OCH TEKNOLOGIERx Materialteknikx Textil-, gummi- och polymermaterial0 (SwePub)205042 hsv//swe |
650 | 7 | a ENGINEERING AND TECHNOLOGYx Materials Engineeringx Textile, Rubber and Polymeric Materials0 (SwePub)205042 hsv//eng |
653 | a morphology | |
653 | a all-polymer solar cells | |
653 | a crystallinity | |
653 | a device performance | |
700 | 1 | a Li, Zhaojun,d 1989u Chalmers tekniska högskola,Chalmers University of Technology4 aut0 (Swepub:cth)zhaojun |
700 | 1 | a Pang, Shutingu South China University of Technology4 aut |
700 | 1 | a Zhu, You-Liangu Chinese Academy of Sciences4 aut |
700 | 1 | a Lin, Baojunu Xi'an Jiaotong University4 aut |
700 | 1 | a Colberts, Fallon J. M.u Technische Universiteit Eindhoven,Eindhoven University of Technology4 aut |
700 | 1 | a Leenaers, Pieter J.u Technische Universiteit Eindhoven,Eindhoven University of Technology4 aut |
700 | 1 | a Wang, Ergang,d 1981u Chalmers tekniska högskola,Chalmers University of Technology4 aut0 (Swepub:cth)ergang |
700 | 1 | a Sun, Zhao-Yanu Chinese Academy of Sciences4 aut |
700 | 1 | a Ma, Weiu Xi'an Jiaotong University4 aut |
700 | 1 | a Meskers, Stefan C. J.u Technische Universiteit Eindhoven,Eindhoven University of Technology4 aut |
700 | 1 | a Janssen, Rene A. J.u Technische Universiteit Eindhoven,Eindhoven University of Technology,Dutch Institute for Fundamental Energy Research (DIFFER)4 aut |
710 | 2 | a Technische Universiteit Eindhovenb South China University of Technology4 org |
773 | 0 | t Solar RRLd : Wileyg 2:12q 2:12x 2367-198X |
856 | 4 | u https://research.chalmers.se/publication/516676/file/516676_Fulltext.pdfx primaryx freey FULLTEXT |
856 | 4 | u https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/solr.201800247 |
856 | 4 8 | u https://doi.org/10.1002/solr.201800247 |
856 | 4 8 | u https://research.chalmers.se/publication/516676 |
856 | 4 8 | u https://research.chalmers.se/publication/507531 |
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