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Atomic-scale visualization of inertial dynamics

Lindenberg, AM (author)
Larsson, Jörgen (author)
Lund University,Lunds universitet,Atomfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Atomic Physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH
Sokolowski-Tinten, K (author)
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Gaffney, KJ (author)
Blome, C (author)
Synnergren, Ola (author)
Lund University,Lunds universitet,Atomfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Atomic Physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH
Sheppard, J (author)
Caleman, C (author)
Uppsala universitet,Institutionen för cell- och molekylärbiologi,Molekylär biofysik
MacPhee, AG (author)
Weinstein, D (author)
Lowney, DP (author)
Allison, TK (author)
Matthews, T (author)
Falcone, RW (author)
Cavalieri, AL (author)
Fritz, DM (author)
Lee, SH (author)
Bucksbaum, PH (author)
Reis, DA (author)
Rudati, J (author)
Fuoss, PH (author)
Kao, CC (author)
Siddons, DP (author)
Pahl, R (author)
Als-Nielsen, J (author)
van der Spoel, D (author)
Uppsala universitet,Institutionen för cell- och molekylärbiologi,Molekylär biofysik
Ischebeck, R (author)
Schlarb, H (author)
Schulte-Schrepping, H (author)
Tschentscher, T (author)
Schneider, J (author)
von der Linde, D (author)
Hignette, O (author)
Sette, F (author)
Chapman, HN (author)
Lee, RW (author)
Timneanu, N (author)
Uppsala universitet,Institutionen för cell- och molekylärbiologi,Molekylär biofysik
Techert, S (author)
Wark, JS (author)
Bergh, M (author)
Uppsala universitet,Institutionen för cell- och molekylärbiologi,Molekylär biofysik
Huldt, G (author)
Uppsala universitet,Institutionen för cell- och molekylärbiologi,Molekylär biofysik
van der Spoel, D (author)
Timneanu, N (author)
Hajdu, J (author)
Uppsala universitet,Institutionen för cell- och molekylärbiologi,Molekylär biofysik
Akre, RA (author)
Bong, E (author)
Krejcik, P (author)
Arthur, J (author)
Brennan, S (author)
Luening, K (author)
Hastings, JB (author)
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 (creator_code:org_t)
American Association for the Advancement of Science (AAAS), 2005
2005
English.
In: Science. - : American Association for the Advancement of Science (AAAS). - 1095-9203 .- 0036-8075. ; 308:5720, s. 392-395
  • Journal article (peer-reviewed)
Abstract Subject headings
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  • The motion of atoms on interatomic potential energy surfaces is fundamental to the dynamics of liquids and solids. An accelerator-based source of femtosecond x-ray pulses allowed us to follow directly atomic displacements on an optically modified energy landscape, leading eventually to the transition from crystalline solid to disordered liquid. We show that, to first order in time, the dynamics are inertial, and we place constraints on the shape and curvature of the transition-state potential energy surface. Our measurements point toward analogies between this nonequilibrium phase transition and the short-time dynamics intrinsic to equilibrium liquids.

Subject headings

NATURVETENSKAP  -- Fysik -- Atom- och molekylfysik och optik (hsv//swe)
NATURAL SCIENCES  -- Physical Sciences -- Atom and Molecular Physics and Optics (hsv//eng)

Publication and Content Type

art (subject category)
ref (subject category)

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