Fuel-rich catalytic combustion of methane in zero emissions power generation processes

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Fältnamn	Indikatorer	Metadata
000		02887naa a2200457 4500
001		oai:DiVA.org:kth-6641
003		SwePub
008		061215s2006 \| \|\|\|\|\|\|\|\|\|\|\|000 \|\|eng\|
024	7	a https://urn.kb.se/resolve?urn=urn:nbn:se:kth:diva-66412 URI
024	7	a https://doi.org/10.1016/j.cattod.2006.06.0102 DOI
040		a (SwePub)kth
041		a engb eng
042		9 SwePub
072	7	a ref2 swepub-contenttype
072	7	a art2 swepub-publicationtype
100	1	a Eriksson, Sarau KTH,Kemiteknik4 aut0 (Swepub:kth)u1ls6ur9
245	1 0	a Fuel-rich catalytic combustion of methane in zero emissions power generation processes
264	1	b Elsevier BV,c 2006
338		a print2 rdacarrier
500		a QC 20110125
520		a A novel catalytic combustion concept for zero emissions power generation has been investigated. Catalysts consisting of Rh supported on ZrO2, Ce-ZrO2 or alpha-Al2O3 were prepared and tested under fuel-rich conditions, i.e. for catalytic partial oxidation (CPO) of methane. The experiments were performed in a subscale gas-turbine reactor operating at 5 bar with exhaust gas-diluted feed mixtures.The catalyst support material was found to influence the light-off temperature significantly, which increased in the following order Rh/Ce-ZrO2 < Rh/ZrO2 < Rh/alpha-Al2O3. The Rh loading, however, only had a minor influence. The high activity of Rh/Ce-ZrO2 is probably related to the high dispersion of Rh on Ce-ZrO2 and the high oxygen mobility of this support compared to pure ZrO2. The formation of hydrogen was also found to increase over the catalyst containing ceria in the support material.
650	7	a TEKNIK OCH TEKNOLOGIERx Kemiteknik0 (SwePub)2042 hsv//swe
650	7	a ENGINEERING AND TECHNOLOGYx Chemical Engineering0 (SwePub)2042 hsv//eng
653		a catalytic combustion
653		a catalytic partial oxidation (CPO) of methane
653		a AZEP
653		a rhodium catalysts
653		a ceria
653		a Chemical engineering
653		a Kemiteknik
700	1	a Wolf, M.4 aut
700	1	a Schneider, A.4 aut
700	1	a Mantzaras, J.4 aut
700	1	a Raimondi, F.4 aut
700	1	a Boutonnet, Magaliu KTH,Kemiteknik4 aut0 (Swepub:kth)u14lus4f
700	1	a Järås, Svenu KTH,Kemiteknik4 aut0 (Swepub:kth)u1ba24kl
710	2	a KTHb Kemiteknik4 org
773	0	t Catalysis Todayd : Elsevier BVg 117:4, s. 447-453q 117:4<447-453x 0920-5861x 1873-4308
856	4	u http://www.sciencedirect.com/science?_ob=ArticleURL&_udi=B6TFG-4KF1HRD-4&_user=4478132&_coverDate=10%2F15%2F2006&_alid=508877380&_rdoc=1&_fmt=summary&_orig=search&_cdi=5226&_sort=d&_docanchor=&view=c&_acct=C000034958&_version=1&_urlVersion=0&_userid=4478132&md5=57f78a3c4c27d471e0da861b57ba016f
856	4 8	u https://urn.kb.se/resolve?urn=urn:nbn:se:kth:diva-6641
856	4 8	u https://doi.org/10.1016/j.cattod.2006.06.010

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Av författaren/redakt...: Eriksson, Sara; Wolf, M.; Schneider, A.; Mantzaras, J.; Raimondi, F.; Boutonnet, Magal ...; visa fler...; Järås, Sven; visa färre...

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