Applying laboratory methods for durability assessment of vitrified material to archaeological samples

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Applying laboratory methods for durability assessment of vitrified material to archaeological samples

Nava-Farias, Lorena (författare): Energy and Environment Directorate, Pacific Northwest National Laboratory, Richland, WA, 99354, USA

Neeway, James J. (författare): Energy and Environment Directorate, Pacific Northwest National Laboratory, Richland, WA, 99354, USA

Schweiger, Michael J. (författare): US Department of Energy, Office of River Protection, Richland, WA, 99352, USA

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Marcial, José (författare): Energy and Environment Directorate, Pacific Northwest National Laboratory, Richland, WA, 99354, USA

Canfield, Nathan L. (författare): Energy and Environment Directorate, Pacific Northwest National Laboratory, Richland, WA, 99354, USA

Pearce, Carolyn I. (författare): Energy and Environment Directorate, Pacific Northwest National Laboratory, Richland, WA, 99354, USA

Peeler, David K. (författare): Energy and Environment Directorate, Pacific Northwest National Laboratory, Richland, WA, 99354, USA

Vicenzi, Edward P. (författare): Smithsonian Institution, Museum Conservation Institute, 4610 Silver Hill Road, Suitland, MD, 20746, USA

Kosson, David S. (författare): School of Engineering, Vanderbilt University, Nashville, TN, 37235, USA

Delapp, Rossane C. (författare): School of Engineering, Vanderbilt University, Nashville, TN, 37235, USA

McCloy, John S. (författare): School of Mechanical and Materials Engineering, Washington State University, Pullman, WA, 99164, USA

Walling, Sam A. (författare): Department of Materials Science & Engineering, The University of Sheffield, Sheffield, S1 3JD, UK

Thorpe, Clare L. (författare): Department of Materials Science & Engineering, The University of Sheffield, Sheffield, S1 3JD, UK

Corkhill, Claire L. (författare): Department of Materials Science & Engineering, The University of Sheffield, Sheffield, S1 3JD, UK

Hand, Russell J. (författare): Department of Materials Science & Engineering, The University of Sheffield, Sheffield, S1 3JD, UK

Sjöblom, Rolf (författare): Luleå tekniska universitet,Geovetenskap och miljöteknik

Kruger, Albert A. (författare): US Department of Energy, Office of River Protection, Richland, WA, 99352, USA

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2021-11-12
2021
Engelska.
Ingår i: npj Materials Degradation. - : Springer Nature. - 2397-2106. ; 5:1

Relaterad länk:: https://doi.org/10.1...; visa fler...; https://www.nature.c...; https://urn.kb.se/re...; https://doi.org/10.1...; visa färre...

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Laboratory testing used to assess the long-term chemical durability of nuclear waste forms may not be applicable to disposal because the accelerated conditions may not represent disposal conditions. To address this, we examine the corrosion of vitrified archeological materials excavated from the near surface of a ~1500-year old Iron Age Swedish hillfort, Broborg, as an analog for the disposal of vitrified nuclear waste. We compare characterized site samples with corrosion characteristics generated by standard laboratory durability test methods including the product consistency test (PCT), the vapor hydration test (VHT), and the EPA Method 1313 test. Results show that the surficial layer of the Broborg samples resulting from VHT displays some similarities to the morphology of the surficial layer formed over longer timescales in the environment. This work provides improved understanding of long-term glass corrosion behavior in terms of the thickness, morphology, and chemistry of the surficial features that are formed.

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Av författaren/redakt...: Nava-Farias, Lor ...; Neeway, James J.; Schweiger, Micha ...; Marcial, José; Canfield, Nathan ...; Pearce, Carolyn ...; visa fler...; Peeler, David K.; Vicenzi, Edward ...; Kosson, David S.; Delapp, Rossane ...; McCloy, John S.; Walling, Sam A.; Thorpe, Clare L.; Corkhill, Claire ...; Hand, Russell J.; Sjöblom, Rolf; Kruger, Albert A ...; visa färre...

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Applying laboratory methods for durability assessment of vitrified material to archaeological samples

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