L773:2198 3844 OR L773:2198 3844
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Solid-State Janus Nanoprecipitation Enables Amorphous-Like Heat Conduction in Crystalline Mg3Sb2-Based Thermoelectric Materials
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- Shu, Rui (author)
- Linköpings universitet,Tunnfilmsfysik,Tekniska fakulteten,Southern Univ Sci & Technol, Peoples R China
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- Han, Zhijia (author)
- Southern Univ Sci & Technol, Peoples R China
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- Elsukova, Anna (author)
- Linköpings universitet,Tunnfilmsfysik,Tekniska fakulteten
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- (creator_code:org_t)
- 2022-07-18
- 2022
- English.
- In: Advanced Science. - : Wiley. - 2198-3844. ; 9:25
- Journal article (peer-reviewed)
Abstract
Subject headings
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- Solid-state precipitation can be used to tailor material properties, ranging from ferromagnets and catalysts to mechanical strengthening and energy storage. Thermoelectric properties can be modified by precipitation to enhance phonon scattering while retaining charge-carrier transmission. Here, unconventional Janus-type nanoprecipitates are uncovered in Mg3Sb1.5Bi0.5 formed by side-by-side Bi- and Ge-rich appendages, in contrast to separate nanoprecipitate formation. These Janus nanoprecipitates result from local comelting of Bi and Ge during sintering, enabling an amorphous-like lattice thermal conductivity. A precipitate size effect on phonon scattering is observed due to the balance between alloy-disorder and nanoprecipitate scattering. The thermoelectric figure-of-merit ZT reaches 0.6 near room temperature and 1.6 at 773 K. The Janus nanoprecipitation can be introduced into other materials and may act as a general property-tailoring mechanism.
Subject headings
- TEKNIK OCH TEKNOLOGIER -- Kemiteknik -- Annan kemiteknik (hsv//swe)
- ENGINEERING AND TECHNOLOGY -- Chemical Engineering -- Other Chemical Engineering (hsv//eng)
Keyword
- atom probe tomography; Janus nanoprecipitation; low thermal conductivity; Mg3Sb2; thermalelectrics
Publication and Content Type
- ref (subject category)
- art (subject category)
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- Shu, Rui
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- Elsukova, Anna
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