Resonant Inelastic X-Ray Scattering Reveals Hidden Local Transitions of the Aqueous OH Radical

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Fältnamn	Indikatorer	Metadata
000		05161naa a2200601 4500
001		oai:DiVA.org:uu-418739
003		SwePub
008		200904s2020 \| \|\|\|\|\|\|\|\|\|\|\|000 \|\|eng\|
024	7	a https://urn.kb.se/resolve?urn=urn:nbn:se:uu:diva-4187392 URI
024	7	a https://doi.org/10.1103/PhysRevLett.124.2360012 DOI
040		a (SwePub)uu
041		a engb eng
042		9 SwePub
072	7	a ref2 swepub-contenttype
072	7	a art2 swepub-publicationtype
100	1	a Kjellsson, Ludvigu Uppsala universitet,Molekyl- och kondenserade materiens fysik4 aut0 (Swepub:uu)ludkj681
245	1 0	a Resonant Inelastic X-Ray Scattering Reveals Hidden Local Transitions of the Aqueous OH Radical
264	1	b AMER PHYSICAL SOC,c 2020
338		a print2 rdacarrier
520		a Resonant inelastic x-ray scattering (RIXS) provides remarkable opportunities to interrogate ultra-fast dynamics in liquids. Here we use RIXS to study the fundamentally and practically important hydroxyl radical in liquid water, OH(aq). Impulsive ionization of pure liquid water produced a short-lived population of OH(aq), which was probed using femtosecond x-rays from an x-ray free-electron laser. We find that RIXS reveals localized electronic transitions that are masked in the ultraviolet absorption spectrum by strong charge-transfer transitions-thus providing a means to investigate the evolving electronic structure and reactivity of the hydroxyl radical in aqueous and heterogeneous environments. First-principles calculations provide interpretation of the main spectral features.
650	7	a NATURVETENSKAPx Kemix Fysikalisk kemi0 (SwePub)104022 hsv//swe
650	7	a NATURAL SCIENCESx Chemical Sciencesx Physical Chemistry0 (SwePub)104022 hsv//eng
650	7	a NATURVETENSKAPx Fysikx Den kondenserade materiens fysik0 (SwePub)103042 hsv//swe
650	7	a NATURAL SCIENCESx Physical Sciencesx Condensed Matter Physics0 (SwePub)103042 hsv//eng
700	1	a Nanda, K. D.u Univ Southern Calif, Dept Chem, Los Angeles, CA 90007 USA.4 aut
700	1	a Rubensson, Jan-Eriku Uppsala universitet,Molekyl- och kondenserade materiens fysik4 aut0 (Swepub:uu)janerube
700	1	a Doumy, G.u Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA.4 aut
700	1	a Southworth, S. H.u Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA.4 aut
700	1	a Ho, P. J.u Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA.4 aut
700	1	a March, A. M.u Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA.4 aut
700	1	a Al Haddad, A.u Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA.4 aut
700	1	a Kumagai, Y.u Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA.4 aut
700	1	a Tu, M-Fu Argonne Natl Lab, Ctr Nanoscale Mat, Lemont, IL 60439 USA.;Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA.4 aut
700	1	a Schaller, R. D.u Argonne Natl Lab, Ctr Nanoscale Mat, Lemont, IL 60439 USA.;Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA.4 aut
700	1	a Debnath, T.u Nanyang Technol Univ, Div Chem & Biol Chem, Singapore 639798, Singapore.4 aut
700	1	a Yusof, M. S. Bin Mohdu Nanyang Technol Univ, Div Chem & Biol Chem, Singapore 639798, Singapore.4 aut
700	1	a Arnold, C.u DESY, Ctr Free Electron Laser Sci, D-22607 Hamburg, Germany.;Univ Hamburg, Dept Phys, D-20146 Hamburg, Germany.;Hamburg Ctr Ultrafast Imaging, D-22607 Hamburg, Germany.4 aut
700	1	a Schlotter, W. F.u SLAC Natl Accelerator Lab, LCLS, Menlo Pk, CA 94025 USA.4 aut
700	1	a Moeller, S.u SLAC Natl Accelerator Lab, LCLS, Menlo Pk, CA 94025 USA.4 aut
700	1	a Coslovich, G.u SLAC Natl Accelerator Lab, LCLS, Menlo Pk, CA 94025 USA.4 aut
700	1	a Koralek, J. D.u SLAC Natl Accelerator Lab, LCLS, Menlo Pk, CA 94025 USA.4 aut
700	1	a Minitti, M. P.u SLAC Natl Accelerator Lab, LCLS, Menlo Pk, CA 94025 USA.4 aut
700	1	a Vidal, M. L.u Tech Univ Denmark, DTU Chem Dept Chem, DK-2800 Lyngby, Denmark.4 aut
700	1	a Simon, M.u Sorbonne Univ, F-75252 Paris 05, France.;CNRS, Lab Chim Phys Matiere & Rayonnement, F-75252 Paris 05, France.4 aut
700	1	a Santra, R.u DESY, Ctr Free Electron Laser Sci, D-22607 Hamburg, Germany.;Univ Hamburg, Dept Phys, D-20146 Hamburg, Germany.;Hamburg Ctr Ultrafast Imaging, D-22607 Hamburg, Germany.4 aut
700	1	a Loh, Z-Hu Nanyang Technol Univ, Div Chem & Biol Chem, Singapore 639798, Singapore.4 aut
700	1	a Coriani, S.u Tech Univ Denmark, DTU Chem Dept Chem, DK-2800 Lyngby, Denmark.4 aut
700	1	a Krylov, A. , I4 aut
700	1	a Young, L.u Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA.;Univ Chicago, Dept Phys, Chicago, IL 60637 USA.;Univ Chicago, James Franck Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA.4 aut
710	2	a Uppsala universitetb Molekyl- och kondenserade materiens fysik4 org
773	0	t Physical Review Lettersd : AMER PHYSICAL SOCg 124:23q 124:23x 0031-9007x 1079-7114
856	4 8	u https://urn.kb.se/resolve?urn=urn:nbn:se:uu:diva-418739
856	4 8	u https://doi.org/10.1103/PhysRevLett.124.236001

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