Yttrium incorporation in Cr2AlC: On the metastable phase formation and decomposition of (Cr,Y)(2)AlC MAX phase thin films

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Fältnamn	Indikatorer	Metadata
000		04474naa a2200565 4500
001		oai:DiVA.org:uu-496945
003		SwePub
008		230222s2023 \| \|\|\|\|\|\|\|\|\|\|\|000 \|\|eng\|
009		oai:DiVA.org:liu-191197
024	7	a https://urn.kb.se/resolve?urn=urn:nbn:se:uu:diva-4969452 URI
024	7	a https://doi.org/10.1111/jace.189312 DOI
024	7	a https://urn.kb.se/resolve?urn=urn:nbn:se:liu:diva-1911972 URI
040		a (SwePub)uud (SwePub)liu
041		a engb eng
042		9 SwePub
072	7	a ref2 swepub-contenttype
072	7	a art2 swepub-publicationtype
100	1	a Azina, Cliou Rhein Westfal TH Aachen, Mat Chem, Kopernikusstr 10, D-52074 Aachen, Germany.4 aut
245	1 0	a Yttrium incorporation in Cr2AlC :b On the metastable phase formation and decomposition of (Cr,Y)(2)AlC MAX phase thin films
264		c 2022-12-27
264	1	b John Wiley & Sons,c 2023
338		a electronic2 rdacarrier
500		a Funding Agencies\|European Unions Horizon 2020 [824096, 892501]; Swedish Foundation for Strategic Research [EM16-0004]; Swedish Research Council [2018-05973, 2019-00191]
520		a Herein we report on the synthesis of a metastable (Cr,Y)(2)AlC MAX phase solid solution by co-sputtering from a composite Cr-Al-C and elemental Y target, at room temperature, followed by annealing. However, direct high-temperature synthesis resulted in multiphase films, as evidenced by X-ray diffraction analyses, room-temperature depositions, followed by annealing to 760 degrees C led to the formation of phase pure (Cr,Y)(2)AlC by diffusion. Higher annealing temperatures caused a decomposition of the metastable phase into Cr2AlC, Y5Al3, and Cr-carbides. In contrast to pure Cr2AlC, the Y-containing phase crystallizes directly in the MAX phase structure instead of first forming a disordered solid solution. Furthermore, the crystallization temperature was shown to be Y-content dependent and was increased by similar to 200 degrees C for 5 at.% Y compared to Cr2AlC. Calculations predicting the metastable phase formation of (Cr,Y)(2)AlC and its decomposition are in excellent agreement with the experimental findings.
650	7	a NATURVETENSKAPx Kemix Materialkemi0 (SwePub)104032 hsv//swe
650	7	a NATURAL SCIENCESx Chemical Sciencesx Materials Chemistry0 (SwePub)104032 hsv//eng
650	7	a NATURVETENSKAPx Kemix Oorganisk kemi0 (SwePub)104042 hsv//swe
650	7	a NATURAL SCIENCESx Chemical Sciencesx Inorganic Chemistry0 (SwePub)104042 hsv//eng
653		a crystallization
653		a decomposition
653		a MAX phases
653		a metastable phase formation
653		a solid solution
700	1	a Bartsch, Timu Rhein Westfal TH Aachen, Mat Chem, Kopernikusstr 10, D-52074 Aachen, Germany.4 aut
700	1	a Holzapfel, Damian M.u Rhein Westfal TH Aachen, Mat Chem, Kopernikusstr 10, D-52074 Aachen, Germany.4 aut
700	1	a Dahlqvist, Martin,d 1982-u Linköpings universitet,Materialdesign,Tekniska fakulteten4 aut0 (Swepub:liu)marda09
700	1	a Rosén, Johanna,c Professor,d 1975-u Linköpings universitet,Materialdesign,Tekniska fakulteten4 aut0 (Swepub:liu)johro07
700	1	a Lofler, Lukasu Rhein Westfal TH Aachen, Mat Chem, Kopernikusstr 10, D-52074 Aachen, Germany.4 aut
700	1	a Mendez, Alba San Joseu Deutsch Elektronen Synchrotron DESY, Hamburg, Germany.4 aut
700	1	a Hans, Marcusu Rhein Westfal TH Aachen, Mat Chem, Kopernikusstr 10, D-52074 Aachen, Germany.4 aut
700	1	a Primetzhofer, Danielu Uppsala universitet,Tillämpad kärnfysik,Uppsala Univ, Sweden4 aut0 (Swepub:uu)danpr521
700	1	a Schneider, Jochen M.u Rhein Westfal TH Aachen, Mat Chem, Kopernikusstr 10, D-52074 Aachen, Germany.4 aut
710	2	a Rhein Westfal TH Aachen, Mat Chem, Kopernikusstr 10, D-52074 Aachen, Germany.b Materialdesign4 org
773	0	t Journal of The American Ceramic Societyd : John Wiley & Sonsg 106:4, s. 2652-2665q 106:4<2652-2665x 0002-7820x 1551-2916
856	4	u https://doi.org/10.1111/jace.18931y Fulltext
856	4	u https://uu.diva-portal.org/smash/get/diva2:1738584/FULLTEXT01.pdfx primaryx Raw objecty fulltext:print
856	4	u https://liu.diva-portal.org/smash/get/diva2:1730388/FULLTEXT01.pdfx primaryx Raw objecty fulltext:print
856	4 8	u https://urn.kb.se/resolve?urn=urn:nbn:se:uu:diva-496945
856	4 8	u https://doi.org/10.1111/jace.18931
856	4 8	u https://urn.kb.se/resolve?urn=urn:nbn:se:liu:diva-191197

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Av författaren/redakt...: Azina, Clio; Bartsch, Tim; Holzapfel, Damia ...; Dahlqvist, Marti ...; Rosén, Johanna, ...; Lofler, Lukas; visa fler...; Mendez, Alba San ...; Hans, Marcus; Primetzhofer, Da ...; Schneider, Joche ...; visa färre...

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