Franck-Condon breakdown in core-level photoelectron spectroscopy of chemisorbed CO

• The photon energy dependence of the vibrational fine structure in the Cls and Ols X-ray photoelectron main lines of chemisorbed CO on Ni(100) and Ru(0001) has been measured from 6 to 150 eV above the core-level thresholds. Significant deviations from the

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VIBRATIONALLY RESOLVED PHOTOELECTRON; MOLECULAR PHOTO-IONIZATION; ANGULAR-DISTRIBUTIONS; SHAPE RESONANCES; THRESHOLD REGION; EXCITED-STATES; PHOTOIONIZATION; PHOTOEMISSION; SPECTRA; CHANNEL

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