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Anti-Stokes resonan...
Anti-Stokes resonant x-ray Raman scattering for atom specific and excited state selective dynamics
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- Kunnus, Kristjan (författare)
- Helmholtz Association of German Research Centers,University of Potsdam
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- Josefsson, Ida (författare)
- Stockholm University,Stockholms universitet,Fysikum
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- Rajkovic, Ivan (författare)
- Max Planck Institute for Biophysical Chemistry
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- Schreck, Simon (författare)
- Stockholm Univ, Dept Phys, AlbaNova Univ Ctr, SE-10691 Stockholm, Sweden,University of Potsdam,Helmholtz Association of German Research Centers
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- Quevedo, Wilson (författare)
- Helmholtz Association of German Research Centers
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- Beye, Martin (författare)
- Helmholtz Association of German Research Centers
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- Grübel, Sebastian (författare)
- Max Planck Institute for Biophysical Chemistry
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- Scholz, Mirko (författare)
- Max Planck Institute for Biophysical Chemistry
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- Nordlund, Dennis (författare)
- Stanford Linear Accelerator Center (SLAC)
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- Zhang, Wenkai (författare)
- Stanford Linear Accelerator Center (SLAC)
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- Hartsock, Robert W. (författare)
- Stanford Linear Accelerator Center (SLAC)
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- Gaffney, Kelly J. (författare)
- Stanford Linear Accelerator Center (SLAC)
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- Schlotter, William F. (författare)
- Stanford Linear Accelerator Center (SLAC)
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- Turner, Joshua J. (författare)
- Stanford Linear Accelerator Center (SLAC)
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- Kennedy, Brian (författare)
- Helmholtz Association of German Research Centers
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- Hennies, Franz (författare)
- Lund University,Lunds universitet,MAX IV-laboratoriet,MAX IV Laboratory
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- Techert, Simone (författare)
- Max Planck Institute for Biophysical Chemistry,University of Göttingen,German Electron Synchrotron (DESY)
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- Wernet, Philippe (författare)
- Helmholtz Association of German Research Centers
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- Odelius, Michael (författare)
- Stockholm University,Stockholms universitet,Fysikum
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- Föhlisch, Alexander (författare)
- University of Potsdam,Helmholtz Association of German Research Centers
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(creator_code:org_t)
- 2016-10-07
- 2016
- Engelska.
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Ingår i: New Journal of Physics. - : IOP Publishing. - 1367-2630. ; 18
- Relaterad länk:
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https://doi.org/10.1...
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https://doi.org/10.1...
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http://dx.doi.org/10... (free)
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https://urn.kb.se/re...
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https://doi.org/10.1...
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https://lup.lub.lu.s...
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Abstract
Ämnesord
Stäng
- Ultrafast electronic and structural dynamics of matter govern rate and selectivity of chemical reactions, as well as phase transitions and efficient switching in functional materials. Since x-rays determine electronic and structural properties with elemental, chemical, orbital and magnetic selectivity, short pulse x-ray sources have become central enablers of ultrafast science. Despite of these strengths, ultrafast x-rays have been poor at picking up excited state moieties from the unexcited ones. With time-resolved anti-Stokes resonant x-ray Raman scattering (AS-RXRS) performed at the LCLS, and ab initio theory we establish background free excited state selectivity in addition to the elemental, chemical, orbital and magnetic selectivity of x-rays. This unparalleled selectivity extracts low concentration excited state species along the pathway of photo induced ligand exchange of Fe(CO)(5) in ethanol. Conceptually a full theoretical treatment of all accessible insights to excited state dynamics with AS-RXRS with transform-limited x-ray pulses is given-which will be covered experimentally by upcoming transform-limited x-ray sources.
Ämnesord
- NATURVETENSKAP -- Fysik (hsv//swe)
- NATURAL SCIENCES -- Physical Sciences (hsv//eng)
- NATURVETENSKAP -- Fysik -- Acceleratorfysik och instrumentering (hsv//swe)
- NATURAL SCIENCES -- Physical Sciences -- Accelerator Physics and Instrumentation (hsv//eng)
Nyckelord
- ultrafast photochemistry
- excited state selectivity
- anti-Stokes resonant x-ray raman scattering
- free electron lasers
- resonant inelastic x-ray scattering
- anti-Stokes resonant x-ray raman scattering
- excited state selectivity
- free electron lasers
- resonant inelastic x-ray scattering
- ultrafast photochemistry
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Till lärosätets databas
- Av författaren/redakt...
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Kunnus, Kristjan
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Josefsson, Ida
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Rajkovic, Ivan
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Schreck, Simon
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Quevedo, Wilson
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Beye, Martin
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visa fler...
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Grübel, Sebastia ...
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Scholz, Mirko
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Nordlund, Dennis
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Zhang, Wenkai
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Hartsock, Robert ...
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Gaffney, Kelly J ...
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Schlotter, Willi ...
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Turner, Joshua J ...
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Kennedy, Brian
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Hennies, Franz
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Techert, Simone
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Wernet, Philippe
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Odelius, Michael
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Föhlisch, Alexan ...
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- NATURVETENSKAP
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NATURVETENSKAP
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- NATURVETENSKAP
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NATURVETENSKAP
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och Fysik
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och Acceleratorfysik ...
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New Journal of P ...
- Av lärosätet
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Stockholms universitet
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Lunds universitet