Sökning: L773:2405 8297 > Insight of electro-...
Fältnamn | Indikatorer | Metadata |
---|---|---|
000 | 04071naa a2200505 4500 | |
001 | oai:research.chalmers.se:e565c770-a4c3-417b-9e88-615f122fdcc9 | |
003 | SwePub | |
008 | 230706s2023 | |||||||||||000 ||eng| | |
024 | 7 | a https://research.chalmers.se/publication/5364382 URI |
024 | 7 | a https://doi.org/10.1016/j.ensm.2023.1028642 DOI |
040 | a (SwePub)cth | |
041 | a engb eng | |
042 | 9 SwePub | |
072 | 7 | a art2 swepub-publicationtype |
072 | 7 | a ref2 swepub-contenttype |
100 | 1 | a Jiao, Xingxingu Xi'an Jiaotong University4 aut |
245 | 1 0 | a Insight of electro-chemo-mechanical process inside integrated configuration of composite cathode for solid-state batteries |
264 | 1 | c 2023 |
520 | a The complicated electro-chemo-mechanical process that occurs inside the composite cathode for solid-state batteries (SSBs), is of first importance to be insighted for the development of SSBs to seek higher energy density. Herein, exampled with layered transition-metal oxide of LiNixCoyMn1-x-yO2 (NCM), an electro-chemo-mechanical model containing electrochemical kinetics, finite-strain constitutive model and cohesive zone model was built to uncover the impact of ionic conductivity and Young's modulus (E) of solid-state electrolyte (SE) on the electro-chemo-mechanical process inside composite cathode and the intergranular failure of single cathode particle. The intergranular failure of NCM particles is powerfully determined by the Young's modulus of SE and the primary particle size, which is postponed by the coarse-primary NCM with soft SE of E=∼2 GPa. Compared with Young's modulus, increasing the ionic conductivity can uniform the distribution of both Li-ion and stress in the whole composite NCM cathode, realizing improved electrochemical performance with larger normalized capacity and lower the interfacial impendence. Hence, high-adequate ionic conductivity of 5 × 10−4 S cm−1 and soft mechanical property of E=∼2 GPa can be proposed as the guideline of SE for great electrochemical performance with prolongated lifespan of composite NCM cathode, paving an avenue to foster the application of SSBs. | |
650 | 7 | a NATURVETENSKAPx Kemix Oorganisk kemi0 (SwePub)104042 hsv//swe |
650 | 7 | a NATURAL SCIENCESx Chemical Sciencesx Inorganic Chemistry0 (SwePub)104042 hsv//eng |
650 | 7 | a TEKNIK OCH TEKNOLOGIERx Maskinteknikx Teknisk mekanik0 (SwePub)203012 hsv//swe |
650 | 7 | a ENGINEERING AND TECHNOLOGYx Mechanical Engineeringx Applied Mechanics0 (SwePub)203012 hsv//eng |
650 | 7 | a NATURVETENSKAPx Kemix Materialkemi0 (SwePub)104032 hsv//swe |
650 | 7 | a NATURAL SCIENCESx Chemical Sciencesx Materials Chemistry0 (SwePub)104032 hsv//eng |
650 | 7 | a TEKNIK OCH TEKNOLOGIERx Materialteknikx Kompositmaterial och -teknik0 (SwePub)205022 hsv//swe |
650 | 7 | a ENGINEERING AND TECHNOLOGYx Materials Engineeringx Composite Science and Engineering0 (SwePub)205022 hsv//eng |
650 | 7 | a NATURVETENSKAPx Fysikx Den kondenserade materiens fysik0 (SwePub)103042 hsv//swe |
650 | 7 | a NATURAL SCIENCESx Physical Sciencesx Condensed Matter Physics0 (SwePub)103042 hsv//eng |
653 | a Electro-chemo-mechanical model | |
653 | a Composite cathode | |
653 | a Intergranular failure | |
653 | a Solid-state electrolyte | |
653 | a Solid-state batteries | |
700 | 1 | a Wang, Yongjingu Xi'an Jiaotong University4 aut |
700 | 1 | a Chen, Yaqiu Xi'an Jiaotong University4 aut |
700 | 1 | a Wang, Jialinu Xi'an Jiaotong University4 aut |
700 | 1 | a Xiong, Shizhao,d 1985u Chalmers tekniska högskola,Chalmers University of Technology4 aut0 (Swepub:cth)xiongs |
700 | 1 | a Song, Zhongxiaou Xi'an Jiaotong University4 aut |
700 | 1 | a Xu, Xieyuu Xi'an Jiaotong University4 aut |
700 | 1 | a Liu, Yangyangu Xi'an Jiaotong University4 aut |
710 | 2 | a Xi'an Jiaotong Universityb Chalmers tekniska högskola4 org |
773 | 0 | t Energy Storage Materialsg 61q 61x 2405-8297 |
856 | 4 8 | u https://research.chalmers.se/publication/536438 |
856 | 4 8 | u https://doi.org/10.1016/j.ensm.2023.102864 |
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