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LIBRIS Formathandbok  (Information om MARC21)
FältnamnIndikatorerMetadata
00004008naa a2200469 4500
001oai:DiVA.org:liu-158547
003SwePub
008190703s2019 | |||||||||||000 ||eng|
024a https://urn.kb.se/resolve?urn=urn:nbn:se:liu:diva-1585472 URI
024a https://doi.org/10.1038/s41467-019-10351-52 DOI
040 a (SwePub)liu
041 a engb eng
042 9 SwePub
072 7a ref2 swepub-contenttype
072 7a art2 swepub-publicationtype
100a Cui, Yongu Chinese Acad Sci, Peoples R China; Univ Chinese Acad Sci, Peoples R China4 aut
2451 0a Over 16% efficiency organic photovoltaic cells enabled by a chlorinated acceptor with increased open-circuit voltages
264 c 2019-06-07
264 1b NATURE PUBLISHING GROUP,c 2019
338 a electronic2 rdacarrier
500 a Funding Agencies|National Natural Science Foundation of China [51961135103, 51673201, 21835006, 91633301, 21805287]; Chinese Academy of Science [XDB12030200, KJZDEW-J01]; Youth Innovation Promotion Association CAS [2018043]; Swedish Energy Agency Energimyndigheten [2016-010174]; Swedish Research Council VR [2018-06048]
520 a Broadening the optical absorption of organic photovoltaic (OPV) materials by enhancing the intramolecular push-pull effect is a general and effective method to improve the power conversion efficiencies of OPV cells. However, in terms of the electron acceptors, the most common molecular design strategy of halogenation usually results in down-shifted molecular energy levels, thereby leading to decreased open-circuit voltages in the devices. Herein, we report a chlorinated non-fullerene acceptor, which exhibits an extended optical absorption and meanwhile displays a higher voltage than its fluorinated counterpart in the devices. This unexpected phenomenon can be ascribed to the reduced non-radiative energy loss (0.206 eV). Due to the simultaneously improved short-circuit current density and open-circuit voltage, a high efficiency of 16.5% is achieved. This study demonstrates that finely tuning the OPV materials to reduce the bandgap-voltage offset has great potential for boosting the efficiency.
650 7a NATURVETENSKAPx Fysikx Annan fysik0 (SwePub)103992 hsv//swe
650 7a NATURAL SCIENCESx Physical Sciencesx Other Physics Topics0 (SwePub)103992 hsv//eng
700a Yao, Huifengu Chinese Acad Sci, Peoples R China4 aut
700a Zhang, Jianqiu Natl Ctr Nanosci and Technol, Peoples R China4 aut
700a Zhang, Taou Chinese Acad Sci, Peoples R China4 aut
700a Wang, Yumingu Linköpings universitet,Biomolekylär och Organisk Elektronik,Tekniska fakulteten4 aut0 (Swepub:liu)yumwa29
700a Hong, Lingu Chinese Acad Sci, Peoples R China; Univ Chinese Acad Sci, Peoples R China4 aut
700a Xian, Kaihuu Chinese Acad Sci, Peoples R China; Univ Chinese Acad Sci, Peoples R China4 aut
700a Xu, Boweiu Chinese Acad Sci, Peoples R China4 aut
700a Zhang, Shaoqingu Chinese Acad Sci, Peoples R China; Univ Sci and Technol Beijing, Peoples R China4 aut
700a Peng, Jingu Organtec Ltd, Peoples R China4 aut
700a Wei, Zhixiangu Natl Ctr Nanosci and Technol, Peoples R China4 aut
700a Gao, Fengu Linköpings universitet,Biomolekylär och Organisk Elektronik,Tekniska fakulteten4 aut0 (Swepub:liu)fenga88
700a Hou, Jianhuiu Chinese Acad Sci, Peoples R China; Univ Chinese Acad Sci, Peoples R China4 aut
710a Chinese Acad Sci, Peoples R China; Univ Chinese Acad Sci, Peoples R Chinab Chinese Acad Sci, Peoples R China4 org
773t Nature Communicationsd : NATURE PUBLISHING GROUPg 10q 10x 2041-1723
856u https://liu.diva-portal.org/smash/get/diva2:1334905/FULLTEXT01.pdfx primaryx Raw objecty fulltext:print
856u https://www.nature.com/articles/s41467-019-10351-5.pdf
8564 8u https://urn.kb.se/resolve?urn=urn:nbn:se:liu:diva-158547
8564 8u https://doi.org/10.1038/s41467-019-10351-5

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