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Reply to Comment on 'Instability of the topological surface state in Bi2Se3 upon deposition of gold'

Polyakov, A. (author)
Max Planck Inst Mikrostrukturphys, Weinberg 2, D-06120 Halle, Germany.
Tusche, C. (author)
Max Planck Inst Mikrostrukturphys, Weinberg 2, D-06120 Halle, Germany.;Forschungszentrum Julich, Peter Grunberg Inst PGI 6, D-52425 Julich, Germany.
Ellguth, M. (author)
Max Planck Inst Mikrostrukturphys, Weinberg 2, D-06120 Halle, Germany.;Johannes Gutenberg Univ Mainz, Inst Phys, Staudingerweg 7, D-55116 Mainz, Germany.
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Crozier, E. D. (author)
Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada.
Mohseni, K. (author)
Max Planck Inst Mikrostrukturphys, Weinberg 2, D-06120 Halle, Germany.
Otrokov, M. M. (author)
Univ Basque Country, CFM, Dept Fis Mat, MPC, San Sebastian 20080, Basque Country, Spain.;Ctr Mixto CSIC UPV EHU, San Sebastian 20080, Basque Country, Spain.;Tomsk State Univ, Tomsk 634050, Russia.;St Petersburg State Univ, St Petersburg 198505, Russia.
Zubizarreta, X. (author)
Max Planck Inst Mikrostrukturphys, Weinberg 2, D-06120 Halle, Germany.
Geilhufe, Matthias (author)
KTH,Nordic Institute for Theoretical Physics NORDITA,Max Planck Inst Mikrostrukturphys, Weinberg 2, D-06120 Halle, Germany.;KTH Royal Inst Technol, Stockholm Ctr Quantum Mat, Nordita, Roslagstullsbacken 23, SE-10691 Stockholm, Sweden.;Stockholm Univ, Roslagstullsbacken 23, SE-10691 Stockholm, Sweden.
Geilhufe, Matthias (author)
Stockholms universitet,Nordiska institutet för teoretisk fysik (Nordita),Max-Planck-Institut für Mikrostrukturphysik, Germany
Chulkov, E. V. (author)
Univ Basque Country, CFM, Dept Fis Mat, MPC, San Sebastian 20080, Basque Country, Spain.;Ctr Mixto CSIC UPV EHU, San Sebastian 20080, Basque Country, Spain.;Tomsk State Univ, Tomsk 634050, Russia.;DIPC, San Sebastian 20018, Basque Country, Spain.
Ernst, A. (author)
Max Planck Inst Mikrostrukturphys, Weinberg 2, D-06120 Halle, Germany.;Johannes Kepler Univ Linz, Inst Theoret Phys, A-4040 Linz, Austria.
Meyerheim, H. L. (author)
Max Planck Inst Mikrostrukturphys, Weinberg 2, D-06120 Halle, Germany.
Parkin, S. S. P. (author)
Max Planck Inst Mikrostrukturphys, Weinberg 2, D-06120 Halle, Germany.
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Max Planck Inst Mikrostrukturphys, Weinberg 2, D-06120 Halle, Germany Max Planck Inst Mikrostrukturphys, Weinberg 2, D-06120 Halle, Germany.;Forschungszentrum Julich, Peter Grunberg Inst PGI 6, D-52425 Julich, Germany. (creator_code:org_t)
American Physical Society, 2018
2018
English.
In: Physical Review B. - : American Physical Society. - 2469-9950 .- 2469-9969. ; 98:13
  • Journal article (peer-reviewed)
Abstract Subject headings
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  • In the Comment on our publication [Phys. Rev. B 95, 180202(R) (2017)], R. A. Gordon claims that our main conclusion is not valid, namely that gold atoms deposited in situ on the (0001) surface of single-crystalline Bi2Se3 reside in substitutional sites, i.e., replacing bismuth atoms within the topmost quintuple layer (QL). Based on x-ray absorption near-edge (XANES) spectra and a re-evaluation of extended x-ray absorption fine structure (EXAFS) data above the Au L-III edge, R. A. Gordon concludes that Au resides in a twofold environment as a result of an interface reaction leading to an Au2S-type local structure, in which gold adopts an Au(I) state and is linearly coordinated by selenium atoms. In this Reply, we will confirm the results published in the original paper and their interpretation that Au atoms reside in the substitutional site.

Subject headings

TEKNIK OCH TEKNOLOGIER  -- Materialteknik (hsv//swe)
ENGINEERING AND TECHNOLOGY  -- Materials Engineering (hsv//eng)
NATURVETENSKAP  -- Fysik (hsv//swe)
NATURAL SCIENCES  -- Physical Sciences (hsv//eng)
NATURVETENSKAP  -- Kemi (hsv//swe)
NATURAL SCIENCES  -- Chemical Sciences (hsv//eng)

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