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Interface-driven seebeck effect in two-dimensional trilayer-stacked PtTe2/MoS2/MoS2 heterostructures via electron-electron interactions

Choi, Jae Won (författare)
Chung Ang Univ, Ctr Berry Curvature Based New Phenomena, Dept Phys, Seoul 06974, South Korea.
Lee, Won-Yong (författare)
Uppsala universitet,Fasta tillståndets elektronik
Kim, Si-Hoo (författare)
Chung Ang Univ, Ctr Berry Curvature Based New Phenomena, Dept Phys, Seoul 06974, South Korea.
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Kang, Min-Sung (författare)
Chung Ang Univ, Ctr Berry Curvature Based New Phenomena, Dept Phys, Seoul 06974, South Korea.
Cho, Jung-Min (författare)
Chung Ang Univ, Ctr Berry Curvature Based New Phenomena, Dept Phys, Seoul 06974, South Korea.
Park, No-Won (författare)
Chung Ang Univ, Ctr Berry Curvature Based New Phenomena, Dept Phys, Seoul 06974, South Korea.
Kwon, Hyeok Jun (författare)
Chung Ang Univ, Ctr Berry Curvature Based New Phenomena, Dept Phys, Seoul 06974, South Korea.
Kim, Yun-Ho (författare)
Chung Ang Univ, Ctr Berry Curvature Based New Phenomena, Dept Phys, Seoul 06974, South Korea.
Kim, Gil-Sung (författare)
Chung Ang Univ, Ctr Berry Curvature Based New Phenomena, Dept Phys, Seoul 06974, South Korea.
Yoon, Young-Gui (författare)
Chung Ang Univ, Ctr Berry Curvature Based New Phenomena, Dept Phys, Seoul 06974, South Korea.
Lee, Sang-Kwon (författare)
Chung Ang Univ, Ctr Berry Curvature Based New Phenomena, Dept Phys, Seoul 06974, South Korea.
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Chung Ang Univ, Ctr Berry Curvature Based New Phenomena, Dept Phys, Seoul 06974, South Korea Fasta tillståndets elektronik (creator_code:org_t)
Elsevier, 2023
2023
Engelska.
Ingår i: Nano Energy. - : Elsevier. - 2211-2855 .- 2211-3282. ; 115
  • Tidskriftsartikel (refereegranskat)
Abstract Ämnesord
Stäng  
  • Two-dimensional (2D) platinum telluride (PtTe2), which is one of the promising metallic transition metal dichalcogenides, has been proven as an essential candidate for electronic devices, magnetic devices, type-II Dirac fermions, topological superconductors, and other optoelectronic applications. However, the formation and thermal transport as important thermoelectric (TE) device applications have not been realized in large-area 2D PtTe2 films due to their semi-metallic properties. Here, we report an innovative approach to enhance the in-plane TE power factors by piling the metallic PtTe2 films on high-resistance (> 10 MO) intrinsic MoS2 films to form bilayer-PtTe2/MoS2 (5 nm/7 nm)//sapphire and trilayer-PtTe2/MoS2/MoS2 (5 nm/7 nm/7 nm)//sapphire heterostructures via wet-transfer stacking method. Such approaches can be achieved by utilizing 2D/2D heterostructure to increase the electron effective mass due to the strong electron-electron interaction at interface under temperature gradient along the samples and ultimately increase Seebeck coefficients via interface-driven Seebeck effect along with a metallic high-conductivity top-PtTe2 films. The trilayer-stacked PtTe2/MoS2/MoS2 heterostructures exhibit an extremely high Seebeck coefficient of 21.6 mu V/K and power factor of similar to 0.2 mW/m.K-2, which are 231 % and similar to 727 %, higher than those of the metallic 5-nm-thick single PtTe2 film on the sapphire substrate, respectively. Our new physics and observation can pave the way toward an effective strategy for understating 2D/2D TMDC heterostructure materials for high Fig.-of-merit TE energy harvesting devices.

Ämnesord

NATURVETENSKAP  -- Fysik -- Den kondenserade materiens fysik (hsv//swe)
NATURAL SCIENCES  -- Physical Sciences -- Condensed Matter Physics (hsv//eng)
NATURVETENSKAP  -- Fysik -- Annan fysik (hsv//swe)
NATURAL SCIENCES  -- Physical Sciences -- Other Physics Topics (hsv//eng)

Nyckelord

Platinum ditelluride
Interface-driven Seebeck effect
Phonon drag
Mott formula
2D heterostructure
Effective mass

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