Versatile Functionalization of Carbon Nanomaterials by Ferrate(VI)

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Fältnamn	Indikatorer	Metadata
000		03411naa a2200577 4500
001		oai:DiVA.org:kth-267989
003		SwePub
008		200401s2020 \| \|\|\|\|\|\|\|\|\|\|\|000 \|\|eng\|
024	7	a https://urn.kb.se/resolve?urn=urn:nbn:se:kth:diva-2679892 URI
024	7	a https://doi.org/10.1007/s40820-019-0353-22 DOI
040		a (SwePub)kth
041		a engb eng
042		9 SwePub
072	7	a ref2 swepub-contenttype
072	7	a art2 swepub-publicationtype
100	1	a Zhou, Y.4 aut
245	1 0	a Versatile Functionalization of Carbon Nanomaterials by Ferrate(VI)
264		c 2020-01-21
264	1	b Springer,c 2020
338		a print2 rdacarrier
500		a QC 20200401
520		a As a high-valent iron compound with Fe in the highest accessible oxidation state, ferrate(VI) brings unique opportunities for a number of areas where chemical oxidation is essential. Recently, it is emerging as a novel oxidizing agent for materials chemistry, especially for the oxidation of carbon materials. However, the reported reactivity in liquid phase (H2SO4 medium) is confusing, which ranges from aggressive to moderate, and even incompetent. Meanwhile, the solid-state reactivity underlying the “dry” chemistry of ferrate(VI) remains poorly understood. Herein, we scrutinize the reactivity of K2FeO4 using fullerene C60 and various nanocarbons as substrates. The results unravel a modest reactivity in liquid phase that only oxidizes the active defects on carbon surface and a powerful oxidizing ability in solid state that can open the inert C=C bonds in carbon lattice. We also discuss respective benefit and limitation of the wet and dry approaches. Our work provides a rational understanding on the oxidizing ability of ferrate(VI) and can guide its application in functionalization/transformation of carbons and also other kinds of materials.[Figure not available: see fulltext.].
650	7	a TEKNIK OCH TEKNOLOGIERx Elektroteknik och elektronikx Annan elektroteknik och elektronik0 (SwePub)202992 hsv//swe
650	7	a ENGINEERING AND TECHNOLOGYx Electrical Engineering, Electronic Engineering, Information Engineeringx Other Electrical Engineering, Electronic Engineering, Information Engineering0 (SwePub)202992 hsv//eng
653		a Carbon nanomaterials
653		a Ferrate(VI)
653		a Oxidation
653		a Reactivity
653		a Carbon
653		a Nanostructured materials
653		a Potassium compounds
653		a Reactivity (nuclear)
653		a Carbon nano-materials
653		a Chemical oxidation
653		a Ferrate
653		a Functionalizations
653		a High-valent irons
653		a Materials chemistry
653		a Oxidizing ability
653		a Solid-state reactivity
653		a Iron compounds
700	1	a Zhang, Z. -Y4 aut
700	1	a Huang, X.4 aut
700	1	a Li, Jiantong,d 1980-u KTH,Elektronik och inbyggda system4 aut0 (Swepub:kth)u1nlco2z
700	1	a Li, T.4 aut
710	2	a KTHb Elektronik och inbyggda system4 org
773	0	t Nano-Micro Lettersd : Springerg 12:1q 12:1x 2311-6706x 2150-5551
856	4	u https://doi.org/10.1007/s40820-019-0353-2y Fulltext
856	4	u https://link.springer.com/content/pdf/10.1007/s40820-019-0353-2.pdf
856	4 8	u https://urn.kb.se/resolve?urn=urn:nbn:se:kth:diva-267989
856	4 8	u https://doi.org/10.1007/s40820-019-0353-2

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Av författaren/redakt...: Zhou, Y.; Zhang, Z. -Y; Huang, X.; Li, Jiantong, 19 ...; Li, T.

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