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Imaging molecular structure through femtosecond photoelectron diffraction on aligned and oriented gas-phase molecules

Boll, Rebecca (author)
Rouzee, Arnaud (author)
Adolph, Marcus (author)
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Anielski, Denis (author)
Aquila, Andrew (author)
Bari, Sadia (author)
Bomme, Cedric (author)
Bostedt, Christoph (author)
Bozek, John D. (author)
Chapman, Henry N. (author)
Christensen, Lauge (author)
Coffee, Ryan (author)
Coppola, Niccola (author)
De, Sankar (author)
Decleva, Piero (author)
Epp, Sascha W. (author)
Erk, Benjamin (author)
Filsinger, Frank (author)
Foucar, Lutz (author)
Gorkhover, Tais (author)
Gumprecht, Lars (author)
Hoemke, Andre (author)
Holmegaard, Lotte (author)
Johnsson, Per (author)
Lund University,Lunds universitet,Atomfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Atomic Physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH
Kienitz, Jens S. (author)
Kierspel, Thomas (author)
Krasniqi, Faton (author)
Kuehnel, Kai-Uwe (author)
Maurer, Jochen (author)
Messerschmidt, Marc (author)
Moshammer, Robert (author)
Mueller, Nele L. M. (author)
Rudek, Benedikt (author)
Savelyev, Evgeny (author)
Schlichting, Ilme (author)
Schmidt, Carlo (author)
Scholz, Frank (author)
Schorb, Sebastian (author)
Schulz, Joachim (author)
Seltmann, Joern (author)
Stener, Mauro (author)
Stern, Stephan (author)
Techert, Simone (author)
Thogersen, Jan (author)
Trippel, Sebastian (author)
Viefhaus, Jens (author)
Vrakking, Marc (author)
Stapelfeldt, Henrik (author)
Kuepper, Jochen (author)
Ullrich, Joachim (author)
Rudenko, Artem (author)
Rolles, Daniel (author)
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 (creator_code:org_t)
2014
2014
English.
In: Faraday Discussions. - : Royal Society of Chemistry (RSC). - 1364-5498. ; 171, s. 57-80
  • Journal article (peer-reviewed)
Abstract Subject headings
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  • This paper gives an account of our progress towards performing femtosecond time-resolved photoelectron diffraction on gas-phase molecules in a pump-probe setup combining optical lasers and an X-ray free-electron laser. We present results of two experiments aimed at measuring photoelectron angular distributions of laser-aligned 1-ethynyl-4-fluorobenzene (C8H5F) and dissociating, laser-aligned 1,4-dibromobenzene (C6H4Br2) molecules and discuss them in the larger context of photoelectron diffraction on gas-phase molecules. We also show how the strong nanosecond laser pulse used for adiabatically laser-aligning the molecules influences the measured electron and ion spectra and angular distributions, and discuss how this may affect the outcome of future time-resolved photoelectron diffraction experiments.

Subject headings

NATURVETENSKAP  -- Fysik -- Atom- och molekylfysik och optik (hsv//swe)
NATURAL SCIENCES  -- Physical Sciences -- Atom and Molecular Physics and Optics (hsv//eng)

Publication and Content Type

art (subject category)
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